Process intensification of <scp> CO <sub>2</sub> </scp> chemical absorption in a conjugated double‐helix cross minichannel absorber

Abstract This paper presents a novel design of miniaturized absorber for carbon capture, featuring a conjugated double‐helix cross (Codohec) multi‐minichannel structure. A lab‐scale Codohec module with four minichannels was fabricated, and chemical absorption experiments were conducted using monoethanolamine (MEA) aqueous solution under varied gas and liquid flowrates and MEA concentration conditions. Flow visualization revealed that the unique Codohec design induces diverse bubble morphologies (e.g., swirling, splitting, switching, collision, and recombination), significantly enhancing the two‐phase mass transfer. Results also demonstrated that the Codohec module achieves a processing capacity of up to kg s −1 while maintaining a high overall mass transfer coefficient of 2.75 s −1 , and with an energy consumption below 4.24 W kg −1 . These findings highlight the potential of miniaturized devices for efficient carbon capture with enhanced mass transfer, high throughput and energy efficiency, offering a promising solution for large‐scale industrial applications.

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Publication Details

Journal
AIChE Journal
Published
2025-08-22
DOI
https://doi.org/10.1002/aic.70055
Primary Topic
Carbon Dioxide Capture Technologies
Type
article
Field-Weighted Citation Impact
0.00

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article

Process intensification of CO 2 chemical absorption in a conjugated double‐helix cross minichannel absorber

Hao Cheng, Dominique Tarlet, Lingaï Luo, Yilin Fan
AIChE Journal
Carbon Dioxide Capture Technologies
article

Process intensification of CO 2 chemical absorption in a conjugated double‐helix cross minichannel absorber

Hao Cheng, Dominique Tarlet, Lingaï Luo, Yilin Fan
article en

Abstract

Abstract This paper presents a novel design of miniaturized absorber for carbon capture, featuring a conjugated double‐helix cross (Codohec) multi‐minichannel structure. A lab‐scale Codohec module with four minichannels was fabricated, and chemical absorption experiments were conducted using monoethanolamine (MEA) aqueous solution under varied gas and liquid flowrates and MEA concentration conditions. Flow visualization revealed that the unique Codohec design induces diverse bubble morphologies (e.g., swirling, splitting, switching, collision, and recombination), significantly enhancing the two‐phase mass transfer. Results also demonstrated that the Codohec module achieves a processing capacity of up to kg s −1 while maintaining a high overall mass transfer coefficient of 2.75 s −1 , and with an energy consumption below 4.24 W kg −1 . These findings highlight the potential of miniaturized devices for efficient carbon capture with enhanced mass transfer, high throughput and energy efficiency, offering a promising solution for large‐scale industrial applications.

AIChE JournalVol. 72(1)
Centre National de la Recherche Scientifique (FR), Laboratoire de Thermique et Energie de Nantes (FR)
China Scholarship Council
Affordable and clean energy
Openalex Percentile: Top 78%
Carbon Dioxide Capture Technologies
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Process intensification of <scp> CO <sub>2</sub> </scp> chemical absorption in a conjugated double‐helix cross minichannel absorber — Hao Cheng, Dominique Tarlet, et al. · AIChE Journal (2025) | TGRS Research Map | TGRS