Hybrid plasmonic coupling through multilayer optimum microcavity based quantum dots random laser

The development of random laser-based devices remains a key challenge due to their low efficiency. This study investigates the performance of multilayered random laser cavities encompassing silver nanoparticles and quantum dots as scatters and gain mediums respectively on silver film coated glass substrate. Polyvinyl alcohol as a spacer layer between gain and scatters enables the engineering of plasmon–exciton couplings; its thickness variation significantly influences the lasing threshold and slope efficiency under protective coating of Polydimethylsiloxane (PDMS). RL wavelength is red shifted from ∼ 636.5 nm to ∼ 645.4 nm under variation of spacer thickness from 0 nm to 137 nm attributed to variation in effective refractive index under the influence of plasmon–exciton interaction which enhanced radiative recombination as well. An optimal spacer thickness of 105 nm assisted in lowering the threshold value to 20 μJ/cm 2 , underscoring improved energy confinement and lasing efficiency under hybrid plasmonic coupling. The power Fourier transform analysis of the random lasing spectra assisted the presented approach. These findings provide a compact strategy for developing wavelength-selective plasmon–exciton hybrid lasing systems in advanced photonic applications. • A simple multilayered planar microcavity RL is developed using Ag NPs, QDs, and a tunable PVA spacer on Ag-coated glass. • Plasmon–exciton coupling through spacer control enables improved lasing efficiency, and thresholds, and spectral tunability. • The low-cost and scalable design paves the way for compact, tunable random lasers for integrated photonics.

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Publication Details

Journal
Journal of Luminescence
Published
2025-08-15
DOI
https://doi.org/10.1016/j.jlumin.2025.121455
Primary Topic
Random lasers and scattering media
Type
article
Field-Weighted Citation Impact
0.00

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article

Hybrid plasmonic coupling through multilayer optimum microcavity based quantum dots random laser

Muhammad Ali Khan, Naeem Iqbal, Anwer Hayat, Junhua Tong et al.
Journal of Luminescence
Random lasers and scattering media
article

Hybrid plasmonic coupling through multilayer optimum microcavity based quantum dots random laser

Muhammad Ali Khan, Naeem Iqbal, Anwer Hayat, Junhua Tong, Tianrui Zhai, Gohar Aziz, Xiaoyu Shi, Zhiyang Xu, Xiaomei Gao, Siqi Chang
article en

Abstract

The development of random laser-based devices remains a key challenge due to their low efficiency. This study investigates the performance of multilayered random laser cavities encompassing silver nanoparticles and quantum dots as scatters and gain mediums respectively on silver film coated glass substrate. Polyvinyl alcohol as a spacer layer between gain and scatters enables the engineering of plasmon–exciton couplings; its thickness variation significantly influences the lasing threshold and slope efficiency under protective coating of Polydimethylsiloxane (PDMS). RL wavelength is red shifted from ∼ 636.5 nm to ∼ 645.4 nm under variation of spacer thickness from 0 nm to 137 nm attributed to variation in effective refractive index under the influence of plasmon–exciton interaction which enhanced radiative recombination as well. An optimal spacer thickness of 105 nm assisted in lowering the threshold value to 20 μJ/cm 2 , underscoring improved energy confinement and lasing efficiency under hybrid plasmonic coupling. The power Fourier transform analysis of the random lasing spectra assisted the presented approach. These findings provide a compact strategy for developing wavelength-selective plasmon–exciton hybrid lasing systems in advanced photonic applications. • A simple multilayered planar microcavity RL is developed using Ag NPs, QDs, and a tunable PVA spacer on Ag-coated glass. • Plasmon–exciton coupling through spacer control enables improved lasing efficiency, and thresholds, and spectral tunability. • The low-cost and scalable design paves the way for compact, tunable random lasers for integrated photonics.

Journal of LuminescenceVol. 287
Westlake University (CN), Beijing University of Technology (CN)
National Natural Science Foundation of China, Natural Science Foundation of Beijing Municipality, Beijing Nova Program
Affordable and clean energy
Openalex Percentile: Top 84%
Random lasers and scattering media
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