Defect-Assisted Photocurrent Generated in Landau-Quantized Graphene/Carbon-Doped <i>h</i>-BN/Graphite van der Waals Tunnel Junctions
Carbon-related defects in carbon-doped hexagonal boron nitride (<i>h</i>-BN:C) have emerged as an ideal material for probing the local electric properties of two-dimensional (2D) materials via defect-assisted tunneling. This study demonstrates the generation of defect-assisted photocurrent in a Landau-quantized monolayer graphene (MLG)/<i>h</i>-BN:C/graphite van der Waals tunnel junction. The photoresponse of the junction was investigated under the cyclotron resonance of MLG, where the energy of the light irradiation coincided with the inter-Landau level (LL) optical transition. We demonstrate photocurrent generation under a specific gate and interlayer bias to satisfy the following conditions: 1) The Fermi energy (<i>E</i><sub>F</sub>) of the MLG is located at the boundary between the quantum Hall states (QHS) and non-QHS. 2) The energy of the LLs below <i>E</i><sub>F</sub> of the MLG coincides with that of the carbon defect in the <i>h</i>-BN barrier. These findings contribute to the development of mid-infrared photodetection and local sensing of cyclotron resonance using defect-assisted tunneling.
Authors
- Tomoki Machida (ORCID: https://orcid.org/0000-0002-1938-7415)
- Takashi Taniguchi (ORCID: https://orcid.org/0000-0002-1467-3105)
- Kenji Watanabe (ORCID: https://orcid.org/0000-0003-3701-8119)
- Yuta Seo (ORCID: https://orcid.org/0009-0007-0510-5556)
- Rai Moriya (ORCID: https://orcid.org/0000-0001-7471-7432)
- Yuki Tsuji
Institutions
- National Institute for Materials Science (JP)
- The University of Tokyo (JP)
Publication Details
- Journal
- Nano Letters
- Published
- 2025-08-19
- DOI
- https://doi.org/10.1021/acs.nanolett.5c03517
- Primary Topic
- Graphene research and applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Tokyo Electron
- Japan Society for the Promotion of Science
- National Institute for Materials Science
- Core Research for Evolutional Science and Technology
- JST-Mirai Program