Quantum spin liquid phases in Kitaev materials

We develop a gauge-invariant renormalized mean-field theory (RMFT) to reliably find the quantum spin liquid (QSL) states and their field response for realistic Kitaev materials under strong magnetic fields and described by the generalized Kitaev J-K-Γ- $${\Gamma }^{{\prime} }$$ model. Remarkably, while our RMFT reproduces previous results based on using more complicated numerical methods, it also predicts several new stable QSL states. In particular, since Kitaev spin liquid (KSL) is no longer a saddle point solution, a new exotic 2-cone state distinct from the KSL is found to describe experimental observations well, and hence should be the candidate state realized in the Kitaev material, α-RuCl3. We further explore the mechanism for the suppression of the observed thermal Hall conductivity at low temperatures within the fermionic framework, and show that the polar-angle dependence of the fermionic gap can distinguish the found 2-cone state from the KSL state in further experiments.

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Publication Details

Journal
npj Quantum Materials
Published
2025-08-16
DOI
https://doi.org/10.1038/s41535-025-00811-1
Citations
1
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
1.26

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article

Quantum spin liquid phases in Kitaev materials

Sungkit Yip, Chung‐Yu Mou, Chung-Hou Chung, Po-Hao Chou
1 citations
npj Quantum Materials
Advanced Condensed Matter Physics
1.26
article

Quantum spin liquid phases in Kitaev materials

Sungkit Yip, Chung‐Yu Mou, Chung-Hou Chung, Po-Hao Chou
article en
1 citations

Abstract

We develop a gauge-invariant renormalized mean-field theory (RMFT) to reliably find the quantum spin liquid (QSL) states and their field response for realistic Kitaev materials under strong magnetic fields and described by the generalized Kitaev J-K-Γ- $${\Gamma }^{{\prime} }$$ model. Remarkably, while our RMFT reproduces previous results based on using more complicated numerical methods, it also predicts several new stable QSL states. In particular, since Kitaev spin liquid (KSL) is no longer a saddle point solution, a new exotic 2-cone state distinct from the KSL is found to describe experimental observations well, and hence should be the candidate state realized in the Kitaev material, α-RuCl3. We further explore the mechanism for the suppression of the observed thermal Hall conductivity at low temperatures within the fermionic framework, and show that the polar-angle dependence of the fermionic gap can distinguish the found 2-cone state from the KSL state in further experiments.

npj Quantum MaterialsVol. 10(1)
National Yang Ming Chiao Tung University (TW), National Tsing Hua University (TW), Institute of Physics, Academia Sinica (TW), Institute of Atomic and Molecular Sciences, Academia Sinica (TW)
Ministry of Education, India, National Science and Technology Council
Openalex Percentile: Top 18%
Advanced Condensed Matter Physics
1.26
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