Multigas TDLAS Detection Based on Variational Mode Decomposition: Frequency Division, Filtering and Interference Noise Removal
Multicomponent gas detection is crucial for industrial and environmental monitoring. In systems based on tunable diode laser absorption spectroscopy (TDLAS), conventional filters with fixed parameters and wide transition bands are unable to effectively separate frequency-adjacent signals or suppress interference fringes, which significantly limits system performance. To address these challenges, we propose the twin-variational mode decomposition demodulation (T-VMD-D) algorithm. This novel approach combines a dual-layer variational mode decomposition architecture with advanced software demodulation techniques, overcoming the inherent limitations of hardware filters. Simulations and experiments demonstrate that the T-VMD-D algorithm achieves significantly higher SNR and robustness in low-interval modulation frequency ranges. At a 100 Hz modulation interval, the algorithm achieves concentration fitting accuracies of 0.9984 (CO<sub>2</sub>) and 0.9982 (CH<sub>4</sub>), with detection limits improved to 6.74 ppm and 504.81 ppb, respectively. These results validate the excellent sensitivity and immunity of the method proposed in this paper for practical multicomponent gas detection applications. By adaptively tuning mode decomposition parameters, the framework can be generalized to detect additional gas species, enhancing its versatility in multicomponent sensing scenarios.
Authors
- Jinguang Lv (ORCID: https://orcid.org/0009-0007-2474-2235)
- He Zhang (ORCID: https://orcid.org/0000-0002-1669-1358)
- Zhipeng Wei (ORCID: https://orcid.org/0000-0002-0492-9365)
- Yixuan Gao (ORCID: https://orcid.org/0000-0003-4694-3955)
- Jilong Tang (ORCID: https://orcid.org/0000-0002-2926-8065)
- Yunping Lan (ORCID: https://orcid.org/0000-0002-5536-4456)
- Yingtian Xu
- Chao Ge (ORCID: https://orcid.org/0009-0001-7154-289X)
- Qin Hu
Institutions
- Changchun University of Science and Technology (CN)
- Jilin University (CN)
- Chinese Academy of Sciences (CN)
- Changchun Institute of Optics, Fine Mechanics and Physics (CN)
- Laser Operations (United States) (US)
- Radiation Oncology Institute (US)
- First Hospital of Jilin University (CN)
- Radiation Oncology Associates (US)
Publication Details
- Journal
- Analytical Chemistry
- Published
- 2025-08-18
- DOI
- https://doi.org/10.1021/acs.analchem.5c03057
- Citations
- 1
- Primary Topic
- Spectroscopy and Laser Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.76
Funders
- Education Department of Jilin Province