Multiferroic coupling in bilayer Janus 3R-CrSCl
Two-dimensional (2D) multiferroics with coupled ferroic orders are attractive for reconfigurable and low-power electronics. Here, we report that bilayer Janus CrSCl—modeled via first-principles calculations—exhibits coexisting intrinsic magnetism, sliding ferroelectricity, and ferrovalley polarization across three stacking configurations. In the S–S stacking, interlayer sliding reverses both electric polarization and valley polarization, while simultaneously switching the total magnetic moment. These reversible and strongly coupled order parameters enable electric- and magnetic-field control of four distinct multiferroic states. Our findings establish Janus CrSCl as a promising platform for field-tunable 2D multiferroics and multifunctional device architectures.
Authors
- Yizhang Wu (ORCID: https://orcid.org/0000-0001-6244-8458)
- Yong Wang (ORCID: https://orcid.org/0000-0001-5085-5312)
- Chi Ding (ORCID: https://orcid.org/0000-0003-2278-7652)
- Yu Zhang (ORCID: https://orcid.org/0000-0001-6987-6754)
- Jie Wang (ORCID: https://orcid.org/0000-0001-7854-9376)
- Xian Zhang (ORCID: https://orcid.org/0000-0003-0681-8201)
- Dingyi Yang
- Miao Wang
Institutions
- Xi'an University of Science and Technology (CN)
- University of North Carolina at Chapel Hill (US)
- Nanjing Agricultural University (CN)
- Nanjing Tech University (CN)
- Xidian University (CN)
- Hohai University (CN)
- Shaanxi Science and Technology Department (CN)
- Applied Physical Sciences (United States) (US)
- Shaanxi University of Science and Technology (CN)
- Nanjing University (CN)
Publication Details
- Journal
- Applied Physics Letters
- Published
- 2025-08-18
- DOI
- https://doi.org/10.1063/5.0288383
- Citations
- 1
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.52
Funders
- National Natural Science Foundation of China
- China Postdoctoral Science Foundation
- National Postdoctoral Program for Innovative Talents
- Fundamental Research Funds for the Central Universities
- Key Research and Development Projects of Shaanxi Province