Multiferroic coupling in bilayer Janus 3R-CrSCl

Two-dimensional (2D) multiferroics with coupled ferroic orders are attractive for reconfigurable and low-power electronics. Here, we report that bilayer Janus CrSCl—modeled via first-principles calculations—exhibits coexisting intrinsic magnetism, sliding ferroelectricity, and ferrovalley polarization across three stacking configurations. In the S–S stacking, interlayer sliding reverses both electric polarization and valley polarization, while simultaneously switching the total magnetic moment. These reversible and strongly coupled order parameters enable electric- and magnetic-field control of four distinct multiferroic states. Our findings establish Janus CrSCl as a promising platform for field-tunable 2D multiferroics and multifunctional device architectures.

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Publication Details

Journal
Applied Physics Letters
Published
2025-08-18
DOI
https://doi.org/10.1063/5.0288383
Citations
1
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.52

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article

Multiferroic coupling in bilayer Janus 3R-CrSCl

Yizhang Wu, Yong Wang, Chi Ding, Yu Zhang et al.
1 citations
Applied Physics Letters
2D Materials and Applications
0.52
article

Multiferroic coupling in bilayer Janus 3R-CrSCl

Yizhang Wu, Yong Wang, Chi Ding, Yu Zhang, Jie Wang, Xian Zhang, Dingyi Yang, Miao Wang
article en
1 citations

Abstract

Two-dimensional (2D) multiferroics with coupled ferroic orders are attractive for reconfigurable and low-power electronics. Here, we report that bilayer Janus CrSCl—modeled via first-principles calculations—exhibits coexisting intrinsic magnetism, sliding ferroelectricity, and ferrovalley polarization across three stacking configurations. In the S–S stacking, interlayer sliding reverses both electric polarization and valley polarization, while simultaneously switching the total magnetic moment. These reversible and strongly coupled order parameters enable electric- and magnetic-field control of four distinct multiferroic states. Our findings establish Janus CrSCl as a promising platform for field-tunable 2D multiferroics and multifunctional device architectures.

Applied Physics LettersVol. 127(7)
Xi'an University of Science and Technology (CN), University of North Carolina at Chapel Hill (US), Nanjing Agricultural University (CN), Nanjing Tech University (CN), Xidian University (CN), Hohai University (CN), Shaanxi Science and Technology Department (CN), Applied Physical Sciences (United States) (US), Shaanxi University of Science and Technology (CN), Nanjing University (CN)
National Natural Science Foundation of China, China Postdoctoral Science Foundation, National Postdoctoral Program for Innovative Talents, Fundamental Research Funds for the Central Universities, Key Research and Development Projects of Shaanxi Province
Openalex Percentile: Top 34%
2D Materials and Applications
0.52
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