Interaction of magnetic fields with spinons in a fractionalized state

The 4d-electron trimer lattice Ba₄Nb₁₋ₓRu₃₊ₓO₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures.

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Publication Details

Journal
npj Quantum Materials
Published
2025-08-08
DOI
https://doi.org/10.1038/s41535-025-00809-9
Citations
1
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
1.26

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article

Interaction of magnetic fields with spinons in a fractionalized state

P. Schlottmann, Rahul Nandkishore, Hengdi Zhao, Gang Cao et al.
1 citations
npj Quantum Materials
Advanced Condensed Matter Physics
1.26
article

Interaction of magnetic fields with spinons in a fractionalized state

P. Schlottmann, Rahul Nandkishore, Hengdi Zhao, Gang Cao, L. E. De Long, Yu Zhang, Tristan R. Cao
article en
1 citations

Abstract

The 4d-electron trimer lattice Ba₄Nb₁₋ₓRu₃₊ₓO₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures.

npj Quantum MaterialsVol. 10(1)
Florida State University (US), University of Kentucky (US), University of Colorado Boulder (US), Laboratory for Atmospheric and Space Physics (US)
National Science Foundation, U.S. Department of Energy, Office of Science, Division of Materials Research, Basic Energy Sciences
Openalex Percentile: Top 19%
Advanced Condensed Matter Physics
1.26
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Interaction of magnetic fields with spinons in a fractionalized state — P. Schlottmann, Rahul Nandkishore, et al. · npj Quantum Materials (2025) | TGRS Research Map | TGRS