Light-controlled strong coupling of optical cavity modes spaced by 200 THz

Cavities have driven significant advances in optical physics and quantum science, with applications ranging from lasers and spectroscopy to quantum information processing, simulation, and metrology. For standard optical cavities, each eigenmode corresponds to a single, well-defined frequency. Here, we present a macroscopic optical Fabry-Pérot cavity whose eigenmodes are coherent superpositions of two frequency modes in the VIS-NIR range. Specifically, we demonstrate strong coupling between 384 THz (780 nm) and 580 THz (516 nm) cavity modes by incorporating an intracavity <i>χ</i>⁽²⁾ crystal driven by a non-resonant optical pump at 1529 nm. Strong coupling enables us to demonstrate frequency conversion with an end-to-end, free-space conversion efficiency of 30(1)%, limited by current cavity design and internal cavity losses. We also demonstrate coupling between distinct spatial modes at the two frequencies, extending coherent control to the spatial basis. In conjunction with improved resonator design and low-loss non-linear crystals, we anticipate a factor of >50 increase in two-mode cooperativity for stronger coupling and near-unity conversion efficiency at low pump powers. This platform opens new avenues for cavity-QED experiments, with potential applications spanning cavity-mediated interactions between distinct atomic species, interconnects for quantum networking and modular computing, and spatially multimode cavity physics.