Quantized optical conductivity of gated and irradiated monolayer Pt<sub>2</sub>HgSe<sub>3</sub>

This study explores the optical conductivity of monolayer jacutingaite (Pt<sub>2</sub>HgSe<sub>3</sub>) under tunable gap parameters induced by both static and dynamic electric fields, focusing on interband and intraband transitions. We analyze the photon energy dependence of the optical response, revealing distinct features: the intraband contribution displays a characteristic Drude-like decay, while the interband response exhibits a sharp onset at a threshold energy, consistent with the presence of an energy gap and underlying phase structure. While the pristine Hall conductivity is negligible, it is significantly enhanced through inversion and time-reversal symmetry breaking, achieved <i>via</i> static and dynamic electric fields, respectively. By tuning the gap parameter, we demonstrate a shift in the onset of interband transitions toward lower and higher photon energies, signaling various topological phase transitions. Our findings highlight the material's tunable optical response, with implications for spintronic and valleytronic applications, and underscore the critical role of the energy gap in governing optical absorption and topological characteristics.

Authors

Institutions

Publication Details

Journal
Physical Chemistry Chemical Physics
Published
2025-01-01
DOI
https://doi.org/10.1039/d5cp01883h
Primary Topic
Chalcogenide Semiconductor Thin Films
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Quantized optical conductivity of gated and irradiated monolayer Pt2HgSe3

Ta T. Tho, Bui D. Hoi
Physical Chemistry Chemical Physics
Chalcogenide Semiconductor Thin Films
article

Quantized optical conductivity of gated and irradiated monolayer Pt2HgSe3

Ta T. Tho, Bui D. Hoi
article en

Abstract

This study explores the optical conductivity of monolayer jacutingaite (Pt<sub>2</sub>HgSe<sub>3</sub>) under tunable gap parameters induced by both static and dynamic electric fields, focusing on interband and intraband transitions. We analyze the photon energy dependence of the optical response, revealing distinct features: the intraband contribution displays a characteristic Drude-like decay, while the interband response exhibits a sharp onset at a threshold energy, consistent with the presence of an energy gap and underlying phase structure. While the pristine Hall conductivity is negligible, it is significantly enhanced through inversion and time-reversal symmetry breaking, achieved <i>via</i> static and dynamic electric fields, respectively. By tuning the gap parameter, we demonstrate a shift in the onset of interband transitions toward lower and higher photon energies, signaling various topological phase transitions. Our findings highlight the material's tunable optical response, with implications for spintronic and valleytronic applications, and underscore the critical role of the energy gap in governing optical absorption and topological characteristics.

Physical Chemistry Chemical PhysicsVol. 27(35)
Hue University (VN), Hanoi University (VN)
Openalex Percentile: Top 81%
Chalcogenide Semiconductor Thin Films
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.