Modulation of photoluminescence in a MoS <sub>2</sub> device through tuning the quantum tunneling effect
Transition metal dichalcogenide (TMD) materials, such as molybdenum disulfide (MoS<sub>2</sub>), have emerged as promising platforms for exploring electrically tunable light-matter interactions, which are critical for designing high-performance photodetector systems. In this study, we investigate the advancements in quantum tunneling MoS<sub>2</sub> field-effect transistors (QT-MoS<sub>2</sub> FETs) and their optoelectronic properties, with a focus on photoresponse behavior and photoluminescence (PL) spectral variations driven by photoinduced tunneling currents through oxide layers. The results demonstrate that tunneling-induced exciton and trion dissociation effects lead to a pronounced blue shift in PL spectral peaks and significant changes in light intensity. Compared to normal MoS<sub>2</sub> FETs, QT-MoS<sub>2</sub> FETs exhibit considerably enhanced PL spectral modulation under applied gate bias, underscoring the critical role of tunneling currents in governing optical responses. This work advances the understanding of 2D material-based optoelectronics and highlights their potential for next-generation photodetector applications.
Authors
- Tilo H. Yang (ORCID: https://orcid.org/0000-0002-7048-9513)
- Wen‐Hao Chang (ORCID: https://orcid.org/0000-0003-4880-6006)
- Bor-Wei Liang
- Ching‐Yuan Su (ORCID: https://orcid.org/0000-0001-9295-7587)
- Yeru Chen
- Yuemei Lan
- Yifan Li (ORCID: https://orcid.org/0000-0003-2543-9741)
- You-Jia Huang
- Ting-Hua Lu
- Ruei-Yu Hsu
Institutions
- National Taiwan Normal University (TW)
- National Central University (TW)
- Massachusetts Institute of Technology (US)
Publication Details
- Journal
- Nanoscale Horizons
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5nh00089k
- Primary Topic
- Neural Networks and Reservoir Computing
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Taiwan University
- National Science and Technology Council