Modulation of photoluminescence in a MoS <sub>2</sub> device through tuning the quantum tunneling effect

Transition metal dichalcogenide (TMD) materials, such as molybdenum disulfide (MoS<sub>2</sub>), have emerged as promising platforms for exploring electrically tunable light-matter interactions, which are critical for designing high-performance photodetector systems. In this study, we investigate the advancements in quantum tunneling MoS<sub>2</sub> field-effect transistors (QT-MoS<sub>2</sub> FETs) and their optoelectronic properties, with a focus on photoresponse behavior and photoluminescence (PL) spectral variations driven by photoinduced tunneling currents through oxide layers. The results demonstrate that tunneling-induced exciton and trion dissociation effects lead to a pronounced blue shift in PL spectral peaks and significant changes in light intensity. Compared to normal MoS<sub>2</sub> FETs, QT-MoS<sub>2</sub> FETs exhibit considerably enhanced PL spectral modulation under applied gate bias, underscoring the critical role of tunneling currents in governing optical responses. This work advances the understanding of 2D material-based optoelectronics and highlights their potential for next-generation photodetector applications.

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Publication Details

Journal
Nanoscale Horizons
Published
2025-01-01
DOI
https://doi.org/10.1039/d5nh00089k
Primary Topic
Neural Networks and Reservoir Computing
Type
article
Field-Weighted Citation Impact
0.00

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article

Modulation of photoluminescence in a MoS 2 device through tuning the quantum tunneling effect

Tilo H. Yang, Wen‐Hao Chang, Bor-Wei Liang, Ching‐Yuan Su et al.
Nanoscale Horizons
Neural Networks and Reservoir Computing
article

Modulation of photoluminescence in a MoS 2 device through tuning the quantum tunneling effect

Tilo H. Yang, Wen‐Hao Chang, Bor-Wei Liang, Ching‐Yuan Su, Yeru Chen, Yuemei Lan, Yifan Li, You-Jia Huang, Ting-Hua Lu, Ruei-Yu Hsu
article en

Abstract

Transition metal dichalcogenide (TMD) materials, such as molybdenum disulfide (MoS<sub>2</sub>), have emerged as promising platforms for exploring electrically tunable light-matter interactions, which are critical for designing high-performance photodetector systems. In this study, we investigate the advancements in quantum tunneling MoS<sub>2</sub> field-effect transistors (QT-MoS<sub>2</sub> FETs) and their optoelectronic properties, with a focus on photoresponse behavior and photoluminescence (PL) spectral variations driven by photoinduced tunneling currents through oxide layers. The results demonstrate that tunneling-induced exciton and trion dissociation effects lead to a pronounced blue shift in PL spectral peaks and significant changes in light intensity. Compared to normal MoS<sub>2</sub> FETs, QT-MoS<sub>2</sub> FETs exhibit considerably enhanced PL spectral modulation under applied gate bias, underscoring the critical role of tunneling currents in governing optical responses. This work advances the understanding of 2D material-based optoelectronics and highlights their potential for next-generation photodetector applications.

Nanoscale HorizonsVol. 10(11)
National Taiwan Normal University (TW), National Central University (TW), Massachusetts Institute of Technology (US)
National Taiwan University, National Science and Technology Council
Openalex Percentile: Top 89%
Neural Networks and Reservoir Computing
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