Electrically-Driven Polarized Nano-Light Sources Based on Suspended Graphene Nanoscrolls

Low-dimensional nanomaterials hold great promise for on-chip light-emitting applications and are expected to profoundly influence the evolution of next-generation photonic chips. Currently, microlasers and light-emitting diodes represent the predominant on-chip integrated light sources. Exploring how to employ low-dimensional materials to realize more miniaturized and controllable light sources remains a key research focus over the past decade. In this work, we demonstrate a high-efficiency nanolight source (NLS) based on graphene nanoscrolls (GNSs), with its emission modulated via an external electric field and device structural design. The GNS NLS features a widely tunable emission spectrum, covering wavelengths from the infrared to the visible range. Besides, we investigated the super-Planckian radiation effect in GNSs, which arises from enhanced absorption in the low-dimensional nanostructure. The theoretical calculations reveal that the absorption coefficient of GNSs in the normal direction is larger than 1, thereby indicating their strong radiative emission according to Kirchhoff's Law of thermal radiation. Furthermore, the emission from GNSs can exhibit fast switching behavior (response time ∼ 75 ms), with the degree of polarization reaching 20% in the visible light range. This work provides important support for the study of the emission characteristics of GNSs and holds profound significance for promoting the development of on-chip integrated NLS technology.

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Publication Details

Journal
ACS Nano
Published
2025-08-15
DOI
https://doi.org/10.1021/acsnano.5c07582
Primary Topic
Thermal Radiation and Cooling Technologies
Type
article
Field-Weighted Citation Impact
0.00

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article

Electrically-Driven Polarized Nano-Light Sources Based on Suspended Graphene Nanoscrolls

Xiao-Yue Fan, Xu Han, Zihao Guo, Jiahao Yan et al.
ACS Nano
Thermal Radiation and Cooling Technologies
article

Electrically-Driven Polarized Nano-Light Sources Based on Suspended Graphene Nanoscrolls

Xiao-Yue Fan, Xu Han, Zihao Guo, Jiahao Yan, Longlong Yang, Yang Chai, Yunyun Dai, Zhipei Sun, Lixin Ge, Zhenyu Sun, Qiang Fu, Yeliang Wang, Taimin Miao, Yuan Bo Huang, Luojun Du, Yongzhi Xie, Yunan Gao, Tongtong Xue, Jing-Han Zhao, Shiqi Yang, Zongjie Shen, Gang Wang, Jiakai Wang, Zhexing Duan, Xia Liu
article en

Abstract

Low-dimensional nanomaterials hold great promise for on-chip light-emitting applications and are expected to profoundly influence the evolution of next-generation photonic chips. Currently, microlasers and light-emitting diodes represent the predominant on-chip integrated light sources. Exploring how to employ low-dimensional materials to realize more miniaturized and controllable light sources remains a key research focus over the past decade. In this work, we demonstrate a high-efficiency nanolight source (NLS) based on graphene nanoscrolls (GNSs), with its emission modulated via an external electric field and device structural design. The GNS NLS features a widely tunable emission spectrum, covering wavelengths from the infrared to the visible range. Besides, we investigated the super-Planckian radiation effect in GNSs, which arises from enhanced absorption in the low-dimensional nanostructure. The theoretical calculations reveal that the absorption coefficient of GNSs in the normal direction is larger than 1, thereby indicating their strong radiative emission according to Kirchhoff's Law of thermal radiation. Furthermore, the emission from GNSs can exhibit fast switching behavior (response time ∼ 75 ms), with the degree of polarization reaching 20% in the visible light range. This work provides important support for the study of the emission characteristics of GNSs and holds profound significance for promoting the development of on-chip integrated NLS technology.

ACS NanoVol. 19(33)
Beijing Institute of Technology (CN), Xinyang Normal University (CN), Hong Kong Polytechnic University (HK), John Brown University (US), Chinese Academy of Sciences (CN), Peking University (CN), Brown University (US), Intelligent Systems Research (United States) (US), Advanced Research Institute (US), Institute of Physics (CN), University of Chinese Academy of Sciences (CN), Southeast University (CN), Ministry of Industry and Information Technology (CN), Aalto University (FI)
National Natural Science Foundation of China, National Key Research and Development Program of China
Openalex Percentile: Top 79%
Thermal Radiation and Cooling Technologies
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