Atmospheric-pressure ion transfer in a gas flow device connected to the UniCell buffer gas cell for superheavy elements chemistry: simulation studies

Abstract Man-made superheavy elements (SHE) are produced as energetic recoils in complete-fusion reactions and need to be thermalized in a gas-filled chamber for chemical studies. The ever-shorter half-lives and decreasing production rates of the elements beyond Fl (atomic number Z = 114)-the heaviest element chemically studied today-require the development of novel techniques for quantitative thermalization and fast extraction efficiency. The Universal high-density gas stopping Cell (UniCell), currently under construction, was proposed to achieve this. Within this work, we propose an Ion Transfer by Gas Flow (ITGF) device, which serves as a UniCell ejector to interface with a gas chromatography detector array for chemical studies. Detailed parameter optimizations, using gas dynamics and Monte Carlo ion-trajectory simulations, promise fast (within a few ms) and highly efficient (up to 100%) ion extraction across a wide mass range. These ions can then be transmitted quantitatively through the ITGF into the high-pressure environment needed for further chemical studies.

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Publication Details

Journal
Nuclear Science and Techniques
Published
2025-07-19
DOI
https://doi.org/10.1007/s41365-025-01772-7
Primary Topic
Mass Spectrometry Techniques and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Atmospheric-pressure ion transfer in a gas flow device connected to the UniCell buffer gas cell for superheavy elements chemistry: simulation studies

J. Ballof, J. Krier, Ch. E. Düllmann, Alexander B. Yakushev et al.
Nuclear Science and Techniques
Mass Spectrometry Techniques and Applications
article

Atmospheric-pressure ion transfer in a gas flow device connected to the UniCell buffer gas cell for superheavy elements chemistry: simulation studies

J. Ballof, J. Krier, Ch. E. Düllmann, Alexander B. Yakushev, Yongli Wei
article en

Abstract

Abstract Man-made superheavy elements (SHE) are produced as energetic recoils in complete-fusion reactions and need to be thermalized in a gas-filled chamber for chemical studies. The ever-shorter half-lives and decreasing production rates of the elements beyond Fl (atomic number Z = 114)-the heaviest element chemically studied today-require the development of novel techniques for quantitative thermalization and fast extraction efficiency. The Universal high-density gas stopping Cell (UniCell), currently under construction, was proposed to achieve this. Within this work, we propose an Ion Transfer by Gas Flow (ITGF) device, which serves as a UniCell ejector to interface with a gas chromatography detector array for chemical studies. Detailed parameter optimizations, using gas dynamics and Monte Carlo ion-trajectory simulations, promise fast (within a few ms) and highly efficient (up to 100%) ion extraction across a wide mass range. These ions can then be transmitted quantitatively through the ITGF into the high-pressure environment needed for further chemical studies.

Nuclear Science and TechniquesVol. 36(10)
GSI Helmholtz Centre for Heavy Ion Research (DE), Johannes Gutenberg University Mainz (DE), Helmholtz Institute Mainz (DE)
Bundesministerium für Bildung und Forschung, GSI Helmholtzzentrum für Schwerionenforschung
Openalex Percentile: Top 82%
Mass Spectrometry Techniques and Applications
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