Coupled lattice-charge-magnetic fluctuations for nonlocal flux mediated pairing in cuprate superconductors

Dynamic charge transfers, or charge flux oscillations, generated by anharmonic phonon coupling, have attracted increasing interest in cuprate superconductors. In this article, a new computational method is developed to analyze such charge fluxes along all atomic bonds for a given material, which unveils a surprising fact that cuprate materials with high superconducting transition temperature show a strong tendency to support global charge flux flows beyond local charge oscillations. Such fluxes further show a strong correlation with both the maximum superconducting transition temperature of different cuprate families and the strong magnetic fluctuations as well. Motivated by these findings, we construct a charge flux model derived from quantum field theory to evaluate the effective interactions mediated by these flux flows. Finally, we discuss the implications of this flux-driven pairing mechanism for the design of new high-Tc superconductors, offering a potential strategy for discovering higher Tc superconductive materials.

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Publication Details

Journal
npj Computational Materials
Published
2025-07-19
DOI
https://doi.org/10.1038/s41524-025-01697-0
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
Field-Weighted Citation Impact
0.00

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article

Coupled lattice-charge-magnetic fluctuations for nonlocal flux mediated pairing in cuprate superconductors

Jianghui Pan, Changkai Luo, Yuchuang Cao, Jiahao Dong et al.
npj Computational Materials
Physics of Superconductivity and Magnetism
article

Coupled lattice-charge-magnetic fluctuations for nonlocal flux mediated pairing in cuprate superconductors

Jianghui Pan, Changkai Luo, Yuchuang Cao, Jiahao Dong, Xi Chen, Xin Li
article en

Abstract

Dynamic charge transfers, or charge flux oscillations, generated by anharmonic phonon coupling, have attracted increasing interest in cuprate superconductors. In this article, a new computational method is developed to analyze such charge fluxes along all atomic bonds for a given material, which unveils a surprising fact that cuprate materials with high superconducting transition temperature show a strong tendency to support global charge flux flows beyond local charge oscillations. Such fluxes further show a strong correlation with both the maximum superconducting transition temperature of different cuprate families and the strong magnetic fluctuations as well. Motivated by these findings, we construct a charge flux model derived from quantum field theory to evaluate the effective interactions mediated by these flux flows. Finally, we discuss the implications of this flux-driven pairing mechanism for the design of new high-Tc superconductors, offering a potential strategy for discovering higher Tc superconductive materials.

npj Computational MaterialsVol. 11(1)
Harvard University (US), Peking University (CN), Institute of Physics (CN), Massachusetts Institute of Technology (US)
Harvard University, Harvard Data Science Initiative, Harvard University, FAS Division of Science, Harvard University
Openalex Percentile: Top 88%
Physics of Superconductivity and Magnetism
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Coupled lattice-charge-magnetic fluctuations for nonlocal flux mediated pairing in cuprate superconductors — Jianghui Pan, Changkai Luo, et al. · npj Computational Materials (2025) | TGRS Research Map | TGRS