Guided mode resonance-driven photoluminescence enhancement and angular emission control in a 2D dielectric photonic lattice

Utilizing fluorescent emitters with precisely designed nanostructures regulates their emission characteristics, which has great potential in light-emitting devices, biosensing, and quantum technologies. In this context, we propose a large area nanostructured design on a flexible polyethylene terephthalate (PET) substrate by patterning it in a square periodic symmetry and coating it with a TiO<sub>2</sub> thin layer to demonstrate cost-effective photoluminescence enhancement and directionality. The proposed design enables a controlled light emission enhancement of about 110 times from the emitter layer over the array through resonance-mediated light confinement. Such mode confinement leads to an increase in the local density of states, which leads to a 100-fold increase in the Purcell factor. Beyond amplification, the polarization-dependent excitation of GMR modes enables directional coupling of photoluminescence into the radiative zeroth-order channel, resulting in well-defined angular emission profiles, as validated by angle-resolved spectroscopy and back focal plane imaging for both transverse electric and transverse magnetic polarization of incident light. The proposed large-area photonic array on a PET substrate offers potential for incorporation into advanced light-emitting optical devices, owing to its scalability and adaptability for practical applications.

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Publication Details

Journal
Nanoscale
Published
2025-01-01
DOI
https://doi.org/10.1039/d5nr02160j
Citations
1
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
0.67

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Guided mode resonance-driven photoluminescence enhancement and angular emission control in a 2D dielectric photonic lattice

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Guided mode resonance-driven photoluminescence enhancement and angular emission control in a 2D dielectric photonic lattice

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article en
1 citations

Abstract

Utilizing fluorescent emitters with precisely designed nanostructures regulates their emission characteristics, which has great potential in light-emitting devices, biosensing, and quantum technologies. In this context, we propose a large area nanostructured design on a flexible polyethylene terephthalate (PET) substrate by patterning it in a square periodic symmetry and coating it with a TiO<sub>2</sub> thin layer to demonstrate cost-effective photoluminescence enhancement and directionality. The proposed design enables a controlled light emission enhancement of about 110 times from the emitter layer over the array through resonance-mediated light confinement. Such mode confinement leads to an increase in the local density of states, which leads to a 100-fold increase in the Purcell factor. Beyond amplification, the polarization-dependent excitation of GMR modes enables directional coupling of photoluminescence into the radiative zeroth-order channel, resulting in well-defined angular emission profiles, as validated by angle-resolved spectroscopy and back focal plane imaging for both transverse electric and transverse magnetic polarization of incident light. The proposed large-area photonic array on a PET substrate offers potential for incorporation into advanced light-emitting optical devices, owing to its scalability and adaptability for practical applications.

NanoscaleVol. 17(32)
Orion Corporation (Finland) (FI), Indian Institute of Technology Delhi (IN), Zayed University (AE)
Department of Science and Technology, Ministry of Science and Technology, India, Ministry of Education, India, Indian Institute of Technology Delhi
Affordable and clean energy
Openalex Percentile: Top 29%
Plasmonic and Surface Plasmon Research
0.67
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