Effect of Magnetic Anisotropy and Gradient‐Induced Dzyaloshinskii‐Moriya Interaction on the Formation of Magnetic Skyrmions

Topological spin textures (e.g., skyrmions) can be stabilized by interfacial Dzyaloshinskii-Moriya interaction (DMI) in the magnetic multilayer, which has been intensively studied. Recently, Bloch-type magnetic skyrmions stabilized by composition gradient-induced DMI (g-DMI) have been observed in 10-nm thick CoPt single layer. However, magnetic anisotropy in gradient-composition engineered CoPt (g-CoPt) films is highly sensitive to both the relative Co/Pt composition and the film thickness, leading to a complex interplay with g-DMI. The stability of skyrmions under the combined influence of magnetic anisotropy and g-DMI is crucial yet remains poorly understood. Here, we condcut a systematic study on the characteristics of magnetic skyrmions as a function of gradient polarity and effective gradient (defined as gradient/thickness) in g-CoPt single layers (thickness of 10-30 nm) using magnetic force microscopy (MFM), bulk magnetometry, and topological Hall effect measurements. Brillouin light scattering spectroscopy confirms that both the sign and magnitude of g-DMI depend on the polarity and amplitude of the composition gradient in g-CoPt films. MFM reveals that skyrmion size and density vary with g-CoPt film thickness, gradient polarity, and applied magnetic field. An increased skyrmion density is observed in samples exhibiting higher magnetic anisotropy, in agreement with micromagnetic simulations and energy barrier calculations.