An end-to-end data analysis framework for real-time detection and source identification of pollution events via e-nose networks

Ambient air pollution contributes to an estimated 4.2 million premature deaths worldwide each year, underscoring the imperative for advanced air quality management tools. In heavily industrialized regions, diffuse fugitive leaks and concentrated stack emissions threaten public health and ecosystems, making real-time monitoring and accurate source apportionment indispensable. To address these challenges, we introduce an end-to-end data analysis framework that employs a distributed network of low-cost electronic noses (e-noses) to deliver spatially and temporally resolved emission monitoring. The real-time, high-resolution outputs of e-noses are deconvoluted into discrete emission events using a chemometric pipeline including principal component analysis (PCA), hierarchical cluster analysis (HCA), and multivariate curve resolution-alternating least squares (MCR-ALS). Each event is then characterized within a 5W attribution schema, which identifies what anomaly was detected, when, and where it occurred, why it arose, and who is responsible for mitigation, thereby creating a searchable database of pollution incidents. By combining real-time, low-cost sensing with robust multivariate analysis and stakeholder-centered reporting, this framework enables transparent emission accountability. In turn, it supports rapid mitigation responses and strengthens regulatory compliance in complex industrial regions.

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Publication Details

Journal
Analytical and Bioanalytical Chemistry
Published
2025-07-24
DOI
https://doi.org/10.1007/s00216-025-06014-8
Citations
1
Primary Topic
Advanced Chemical Sensor Technologies
Type
article
Field-Weighted Citation Impact
0.67
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article

An end-to-end data analysis framework for real-time detection and source identification of pollution events via e-nose networks

Jeroen J. Jansen, S. Bootsma, Mahsa Akbari Lakeh, Gerjen H. Tinnevelt et al.
1 citations
Analytical and Bioanalytical Chemistry
Advanced Chemical Sensor Technologies
0.67
article

An end-to-end data analysis framework for real-time detection and source identification of pollution events via e-nose networks

Jeroen J. Jansen, S. Bootsma, Mahsa Akbari Lakeh, Gerjen H. Tinnevelt, Ralph van Nellestijn
article en
1 citations

Abstract

Ambient air pollution contributes to an estimated 4.2 million premature deaths worldwide each year, underscoring the imperative for advanced air quality management tools. In heavily industrialized regions, diffuse fugitive leaks and concentrated stack emissions threaten public health and ecosystems, making real-time monitoring and accurate source apportionment indispensable. To address these challenges, we introduce an end-to-end data analysis framework that employs a distributed network of low-cost electronic noses (e-noses) to deliver spatially and temporally resolved emission monitoring. The real-time, high-resolution outputs of e-noses are deconvoluted into discrete emission events using a chemometric pipeline including principal component analysis (PCA), hierarchical cluster analysis (HCA), and multivariate curve resolution-alternating least squares (MCR-ALS). Each event is then characterized within a 5W attribution schema, which identifies what anomaly was detected, when, and where it occurred, why it arose, and who is responsible for mitigation, thereby creating a searchable database of pollution incidents. By combining real-time, low-cost sensing with robust multivariate analysis and stakeholder-centered reporting, this framework enables transparent emission accountability. In turn, it supports rapid mitigation responses and strengthens regulatory compliance in complex industrial regions.

Analytical and Bioanalytical ChemistryVol. 417(25)
Radboud University Nijmegen (NL), Radboud University Medical Center (NL), Radboud Institute for Molecular Life Sciences (NL), J.M. Burgerscentrum (NL)
Openalex Percentile: Top 29%
Advanced Chemical Sensor Technologies
0.67
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An end-to-end data analysis framework for real-time detection and source identification of pollution events via e-nose networks — Jeroen J. Jansen, S. Bootsma, et al. · Analytical and Bioanalytical Chemistry (2025) | TGRS Research Map | TGRS