Dynamics of conducting ferroelectric domain walls

We report on the dynamics of a conducting domain wall under applied dc and ac voltages. These dynamics are modeled for a thin film that hosts an ideal charged domain wall via a combination of time-dependent Ginzburg-Landau equations for the polarization, the Schrödinger equation for the electron gas, and Poisson's equation for the electrostatic potential. The electron dynamics are treated within a Born-Oppenheimer approximation. We find that the electron gas introduces an additional degree of freedom, beyond polarization relaxation, that modifies the dynamical response of the domain wall. While marginally relevant for the dc response, the electron dynamics have a pronounced effect on the film's ac dielectric function. The dielectric function has an intrinsic contribution, due to the bulk susceptibility of the film, and an extrinsic contribution due to the domain-wall displacement. The elecron gas affects the dielectric function by changing both the amplitude and phase of the displacement.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-07-16
DOI
https://doi.org/10.1103/v293-1x2y
Primary Topic
Solid-state spectroscopy and crystallography
Type
article
Field-Weighted Citation Impact
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article

Dynamics of conducting ferroelectric domain walls

W. A. Atkinson, Karl J. Friston
3 links
Physical review. B./Physical review. B
Solid-state spectroscopy and crystallography
article

Dynamics of conducting ferroelectric domain walls

W. A. Atkinson, Karl J. Friston
article en

Abstract

We report on the dynamics of a conducting domain wall under applied dc and ac voltages. These dynamics are modeled for a thin film that hosts an ideal charged domain wall via a combination of time-dependent Ginzburg-Landau equations for the polarization, the Schrödinger equation for the electron gas, and Poisson's equation for the electrostatic potential. The electron dynamics are treated within a Born-Oppenheimer approximation. We find that the electron gas introduces an additional degree of freedom, beyond polarization relaxation, that modifies the dynamical response of the domain wall. While marginally relevant for the dc response, the electron dynamics have a pronounced effect on the film's ac dielectric function. The dielectric function has an intrinsic contribution, due to the bulk susceptibility of the film, and an extrinsic contribution due to the domain-wall displacement. The elecron gas affects the dielectric function by changing both the amplitude and phase of the displacement.

Physical review. B./Physical review. BVol. 112(2)
Trent University (CA)
Openalex Percentile: Top 88%
Solid-state spectroscopy and crystallography
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