Multi-anion high-entropy electrolytes enabling lithium-ion batteries with enhanced voltage tolerance and wide-temperature operability

To achieve high-voltage stability and low-temperature performance simultaneously in lithium-ion batteries, a high-entropy electrolyte with multi anions is proposed. The multi anions not only lows the solvation-free energy, but also contributes to the formation of inorganic-rich CEI layer. The optimized electrolyte enables stable cycling of NCM523 at both 25 °C and -20 °C.

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Publication Details

Journal
RSC Advances
Published
2025-01-01
DOI
https://doi.org/10.1039/d5ra02919h
Citations
3
Primary Topic
Advancements in Battery Materials
Type
article
Field-Weighted Citation Impact
2.19

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Multi-anion high-entropy electrolytes enabling lithium-ion batteries with enhanced voltage tolerance and wide-temperature operability

Fu‐Da Yu, Jijun Zhao, Lan‐Fang Que, Jihuai Wu et al.
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RSC Advances
Advancements in Battery Materials
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article

Multi-anion high-entropy electrolytes enabling lithium-ion batteries with enhanced voltage tolerance and wide-temperature operability

Fu‐Da Yu, Jijun Zhao, Lan‐Fang Que, Jihuai Wu, Zhang Lan, Hainan Wang, Yiming Xie
article en
3 citations

Abstract

To achieve high-voltage stability and low-temperature performance simultaneously in lithium-ion batteries, a high-entropy electrolyte with multi anions is proposed. The multi anions not only lows the solvation-free energy, but also contributes to the formation of inorganic-rich CEI layer. The optimized electrolyte enables stable cycling of NCM523 at both 25 °C and -20 °C.

RSC AdvancesVol. 15(31)
Huaqiao University (CN)
Natural Science Foundation of Xiamen City, National Natural Science Foundation of China, Natural Science Foundation of Fujian Province, Harbin Institute of Technology, Fundamental Research Funds for the Central Universities
Affordable and clean energy
Openalex Percentile: Top 12%
Advancements in Battery Materials
2.19
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