Observation of Strong Nonreciprocal Thermal Emission

The Kirchhoff's law of thermal radiation stating the equivalence of emissivity and absorptivity at the same wavelength, angle, and polarization, has completely constrained emission and absorption processes. Achieving strong nonreciprocal emission points to fundamental advances for applications such as energy harvesting, heat transfer, and sensing, but strong nonreciprocal thermal emission has not been experimentally realized. Here, we observe strong nonreciprocal thermal emission using a custom-designed angle-resolved magnetic thermal emission spectroscopy and an epitaxially transferred gradient-doped metamaterial. We show that under magnetic field, the metamaterial strongly breaks Kirchhoff's law, with a difference between emissivity and absorptivity at the same wavelength and angle reaching as high as 0.43. Significant nonreciprocal emission persists over broad spectral and angular ranges. The demonstration of strong nonreciprocal thermal emission and the approach can be useful for systematic exploration of nonreciprocal thermal photonics for thermal management, infrared camouflage, and energy conversion.

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Publication Details

Journal
Physical Review Letters
Published
2025-06-30
DOI
https://doi.org/10.1103/physrevlett.135.016901
Citations
16
Primary Topic
Thermal Radiation and Cooling Technologies
Type
article
Field-Weighted Citation Impact
15.25

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article

Observation of Strong Nonreciprocal Thermal Emission

Zhenong Zhang, Linxiao Zhu, Prasanta Ghosh, Alireza Kalantari Dehaghi
16 citations
Physical Review Letters
Thermal Radiation and Cooling Technologies
15.25
article

Observation of Strong Nonreciprocal Thermal Emission

Zhenong Zhang, Linxiao Zhu, Prasanta Ghosh, Alireza Kalantari Dehaghi
article en
16 citations

Abstract

The Kirchhoff's law of thermal radiation stating the equivalence of emissivity and absorptivity at the same wavelength, angle, and polarization, has completely constrained emission and absorption processes. Achieving strong nonreciprocal emission points to fundamental advances for applications such as energy harvesting, heat transfer, and sensing, but strong nonreciprocal thermal emission has not been experimentally realized. Here, we observe strong nonreciprocal thermal emission using a custom-designed angle-resolved magnetic thermal emission spectroscopy and an epitaxially transferred gradient-doped metamaterial. We show that under magnetic field, the metamaterial strongly breaks Kirchhoff's law, with a difference between emissivity and absorptivity at the same wavelength and angle reaching as high as 0.43. Significant nonreciprocal emission persists over broad spectral and angular ranges. The demonstration of strong nonreciprocal thermal emission and the approach can be useful for systematic exploration of nonreciprocal thermal photonics for thermal management, infrared camouflage, and energy conversion.

Physical Review LettersVol. 135(1)
Pennsylvania State University (US)
National Science Foundation, Pittsburgh Foundation, Charles E. Kaufman Foundation, Institutes of Energy and the Environment, Pennsylvania State University
Openalex Percentile: Top 1%
Thermal Radiation and Cooling Technologies
15.25
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