Modulation of Single Photon Emission from Suspended 1L WSe<sub>2</sub> under Electrostatically Induced Strain

Tungsten diselenide (WSe<sub>2</sub>) monolayers under strain are promising hosts for quantum emitters. To date, WSe<sub>2</sub> quantum emitter strain engineering has focused primarily on draping WSe<sub>2</sub> monolayers on patterned substrates and nanoindentation, which suffer from poor control over strain. In this work, we employ an electrostatic approach to dynamically control tensile strain in monolayer WSe<sub>2</sub> suspended over micron-scale cavities with a back gate contact. Room-temperature measurement of electrostatically induced deflection and photoluminescence at <i>T</i> = 100 K shows that a 0.22-0.26% increase in tensile strain can be achieved at modest gate voltages. Sharp localized emitters showed improvement in single photon purity from g<sup>(2)</sup>(0) = 0.55 ± 0.04 at 0 V to g<sup>(2)</sup>(0) = 0.40 ± 0.05 at -30 V due to strain-induced alignment of defect and dark exciton states and classical light background suppression.

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Publication Details

Journal
Nano Letters
Published
2025-06-30
DOI
https://doi.org/10.1021/acs.nanolett.5c02619
Citations
2
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
1.04
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article

Modulation of Single Photon Emission from Suspended 1L WSe2 under Electrostatically Induced Strain

Frances Camille M. Wu, Jean Anne C. Incorvia, Edward T. Yu, Bin Fang et al.
2 citations
Nano Letters
2D Materials and Applications
1.04
article

Modulation of Single Photon Emission from Suspended 1L WSe2 under Electrostatically Induced Strain

Frances Camille M. Wu, Jean Anne C. Incorvia, Edward T. Yu, Bin Fang, Jingxu Kent Zheng, Shang‐Hsuan Wu, Xintong Li
article en
2 citations

Abstract

Tungsten diselenide (WSe<sub>2</sub>) monolayers under strain are promising hosts for quantum emitters. To date, WSe<sub>2</sub> quantum emitter strain engineering has focused primarily on draping WSe<sub>2</sub> monolayers on patterned substrates and nanoindentation, which suffer from poor control over strain. In this work, we employ an electrostatic approach to dynamically control tensile strain in monolayer WSe<sub>2</sub> suspended over micron-scale cavities with a back gate contact. Room-temperature measurement of electrostatically induced deflection and photoluminescence at <i>T</i> = 100 K shows that a 0.22-0.26% increase in tensile strain can be achieved at modest gate voltages. Sharp localized emitters showed improvement in single photon purity from g<sup>(2)</sup>(0) = 0.55 ± 0.04 at 0 V to g<sup>(2)</sup>(0) = 0.40 ± 0.05 at -30 V due to strain-induced alignment of defect and dark exciton states and classical light background suppression.

Nano LettersVol. 25(27)
The University of Texas at Austin (US)
Openalex Percentile: Top 24%
2D Materials and Applications
1.04
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