Modulation of Single Photon Emission from Suspended 1L WSe<sub>2</sub> under Electrostatically Induced Strain
Tungsten diselenide (WSe<sub>2</sub>) monolayers under strain are promising hosts for quantum emitters. To date, WSe<sub>2</sub> quantum emitter strain engineering has focused primarily on draping WSe<sub>2</sub> monolayers on patterned substrates and nanoindentation, which suffer from poor control over strain. In this work, we employ an electrostatic approach to dynamically control tensile strain in monolayer WSe<sub>2</sub> suspended over micron-scale cavities with a back gate contact. Room-temperature measurement of electrostatically induced deflection and photoluminescence at <i>T</i> = 100 K shows that a 0.22-0.26% increase in tensile strain can be achieved at modest gate voltages. Sharp localized emitters showed improvement in single photon purity from g<sup>(2)</sup>(0) = 0.55 ± 0.04 at 0 V to g<sup>(2)</sup>(0) = 0.40 ± 0.05 at -30 V due to strain-induced alignment of defect and dark exciton states and classical light background suppression.
Authors
- Frances Camille M. Wu (ORCID: https://orcid.org/0000-0002-8114-203X)
- Jean Anne C. Incorvia (ORCID: https://orcid.org/0000-0002-4805-2112)
- Edward T. Yu (ORCID: https://orcid.org/0000-0001-9900-7322)
- Bin Fang (ORCID: https://orcid.org/0000-0003-4137-3404)
- Jingxu Kent Zheng (ORCID: https://orcid.org/0000-0002-0673-0560)
- Shang‐Hsuan Wu (ORCID: https://orcid.org/0000-0001-9934-7765)
- Xintong Li (ORCID: https://orcid.org/0000-0001-8566-0558)
Institutions
- The University of Texas at Austin (US)
Publication Details
- Journal
- Nano Letters
- Published
- 2025-06-30
- DOI
- https://doi.org/10.1021/acs.nanolett.5c02619
- Citations
- 2
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 1.04