Phase evolution of strong-field ionization

We investigate the time-dependent evolution of the dipole phase shift induced by strong-field ionization (SFI) using attosecond transient absorption spectroscopy (ATAS) for time delays where the pump-probe pulses overlap. We study measured and calculated time-dependent attosecond transient absorption spectra of the ionic <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:mn>4</a:mn><a:mi mathvariant="italic">d</a:mi><a:mo>→</a:mo><a:mn>5</a:mn><a:mi mathvariant="italic">p</a:mi></a:mrow></a:math> in xenon, and present the time-dependent line shape parameters in the complex plane. We attribute the complex dynamics to the contribution of three distinct processes: accumulation of ionization, transient population, and retrapping of excited states arising from polarization of the ground state.

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Publication Details

Journal
Physical Review Research
Published
2025-06-24
DOI
https://doi.org/10.1103/physrevresearch.7.l022074
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Phase evolution of strong-field ionization

A. C. Brown, Maximilian Hartmann, Shuyuan Hu, Thomas Pfeifer et al.
Physical Review Research
Laser-Matter Interactions and Applications
article

Phase evolution of strong-field ionization

A. C. Brown, Maximilian Hartmann, Shuyuan Hu, Thomas Pfeifer, H. W. van der Hart, Lynda Hutcheson, Paul Birk, Gergana D. Borisova, Christian Ott
article en

Abstract

We investigate the time-dependent evolution of the dipole phase shift induced by strong-field ionization (SFI) using attosecond transient absorption spectroscopy (ATAS) for time delays where the pump-probe pulses overlap. We study measured and calculated time-dependent attosecond transient absorption spectra of the ionic <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:mn>4</a:mn><a:mi mathvariant="italic">d</a:mi><a:mo>→</a:mo><a:mn>5</a:mn><a:mi mathvariant="italic">p</a:mi></a:mrow></a:math> in xenon, and present the time-dependent line shape parameters in the complex plane. We attribute the complex dynamics to the contribution of three distinct processes: accumulation of ionization, transient population, and retrapping of excited states arising from polarization of the ground state.

Physical Review ResearchVol. 7(2)
Queen's University Belfast (GB), Max Planck Institute for Nuclear Physics (DE)
Deutsche Forschungsgemeinschaft, Engineering and Physical Sciences Research Council, H2020 European Research Council
Openalex Percentile: Top 89%
Laser-Matter Interactions and Applications
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Phase evolution of strong-field ionization — A. C. Brown, Maximilian Hartmann, et al. · Physical Review Research (2025) | TGRS Research Map | TGRS