A direct and theoretically consistent method for the calculation of the settling speed of prolate spheroidal particles in the atmosphere

We propose a new method for calculating the settling speed of aerosol particles with prolate shape in the atmosphere. This method takes into account the known theoretical results on the speed-force relationships for prolate spheroids moving in a fluid, and the results in Mallios et al. (2021) regarding the orientation of prolate particles settling in the atmosphere. Unlike other studies, we focus not on the resistance problem (calculating the aerodynamic force as a function of speed) but on the mobility problem (calculate terminal velocity as a function of the external force). The result of this approach is a set of equations that permit to directly calculate the settling speed of a prolate particle in the atmosphere as a function of its shape and characteristics, which is a very important quantity in atmospheric science since the settling speed of a falling particle is a key factor to determine its lifetime in the atmosphere. With this approach, we show that the settling speed is reduced by up to 20% for particles with aspect ratio 4 compared to same-volume spheres. We compare the results of the present study to CFD results of Sanjeevi et al. (2022) and to laboratory measurements of Bhowmick et al. (2024), the latter comparison showing that the estimates for settling speed from our method is within ± 5 % compared to the measured value. Finally, since calculating the terminal speed of settling particles is an important issue in atmospheric modelling, we provide a Fortran module implementing the method described in the present study. • We propose a new method to calculate the settling speed of prolate spheroidal particles in the atmosphere. • This method respects known theoretical results for both spherical and prolate spheroidal particles in the Stokes regime, yet reproduces experimental and CFD results with excellent accuracy for all relevant sizes of aerosol particles in the atmosphere up for particle sizes up to several hundred micrometers. • The effect of non-sphericity on the settling speed of prolate particles in the air is more prononced for coarse particles than for fine particles, reducing settling speed by ≃ 10 % for particles with aspect ratio 2, and by ≃ 20 % for aspect ratio 4. • We have developed and we distribute a Fortran implementation of this method, with a focus on computational efficiency, in order to facilitate its implementation in chemistry-transport models.

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Publication Details

Journal
Journal of Aerosol Science
Published
2025-06-22
DOI
https://doi.org/10.1016/j.jaerosci.2025.106613
Primary Topic
Particle Dynamics in Fluid Flows
Type
article
Field-Weighted Citation Impact
0.00

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article

A direct and theoretically consistent method for the calculation of the settling speed of prolate spheroidal particles in the atmosphere

Sylvain Mailler, Sotirios A. Mallios
Journal of Aerosol Science
Particle Dynamics in Fluid Flows
article

A direct and theoretically consistent method for the calculation of the settling speed of prolate spheroidal particles in the atmosphere

Sylvain Mailler, Sotirios A. Mallios
article en

Abstract

We propose a new method for calculating the settling speed of aerosol particles with prolate shape in the atmosphere. This method takes into account the known theoretical results on the speed-force relationships for prolate spheroids moving in a fluid, and the results in Mallios et al. (2021) regarding the orientation of prolate particles settling in the atmosphere. Unlike other studies, we focus not on the resistance problem (calculating the aerodynamic force as a function of speed) but on the mobility problem (calculate terminal velocity as a function of the external force). The result of this approach is a set of equations that permit to directly calculate the settling speed of a prolate particle in the atmosphere as a function of its shape and characteristics, which is a very important quantity in atmospheric science since the settling speed of a falling particle is a key factor to determine its lifetime in the atmosphere. With this approach, we show that the settling speed is reduced by up to 20% for particles with aspect ratio 4 compared to same-volume spheres. We compare the results of the present study to CFD results of Sanjeevi et al. (2022) and to laboratory measurements of Bhowmick et al. (2024), the latter comparison showing that the estimates for settling speed from our method is within ± 5 % compared to the measured value. Finally, since calculating the terminal speed of settling particles is an important issue in atmospheric modelling, we provide a Fortran module implementing the method described in the present study. • We propose a new method to calculate the settling speed of prolate spheroidal particles in the atmosphere. • This method respects known theoretical results for both spherical and prolate spheroidal particles in the Stokes regime, yet reproduces experimental and CFD results with excellent accuracy for all relevant sizes of aerosol particles in the atmosphere up for particle sizes up to several hundred micrometers. • The effect of non-sphericity on the settling speed of prolate particles in the air is more prononced for coarse particles than for fine particles, reducing settling speed by ≃ 10 % for particles with aspect ratio 2, and by ≃ 20 % for aspect ratio 4. • We have developed and we distribute a Fortran implementation of this method, with a focus on computational efficiency, in order to facilitate its implementation in chemistry-transport models.

Journal of Aerosol ScienceVol. 189
Centre National de la Recherche Scientifique (FR), École Polytechnique (FR), École nationale des ponts et chaussées (FR), Université Paris Sciences et Lettres (FR), École Normale Supérieure - PSL (FR), Sorbonne Université (FR), National Observatory of Athens (GR)
Agence de l'Environnement et de la Maîtrise de l'Energie
Climate action
Openalex Percentile: Top 82%
Particle Dynamics in Fluid Flows
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