Spatiotemporal evolution in femtosecond second-harmonic generation with back-conversion

We systematically investigate second-harmonic generation (SHG) in a lithium triborate (LBO) crystal by a femtosecond laser system (1030 nm, 195 fs, 30 W) with particular emphasis on back-conversion phenomena. For a selected 5 mm thick crystal, an optimal conversion efficiency of 54% is achieved at 18 W input power with beam quality factor M<sup>2</sup> of 1.275 (horizontal) and 1.173 (vertical). Beyond the saturation threshold where back-conversion initiates, spectral broadening, temporal compression and beam quality deterioration emerge, accompanied by decreasing conversion efficiency. Increasing the beam diameter or reducing the crystal length effectively mitigates back-conversion phenomena. These findings establish valuable guidelines for optimizing the performance of femtosecond visible laser sources.

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Publication Details

Journal
Optics Express
Published
2025-06-17
DOI
https://doi.org/10.1364/oe.566024
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Spatiotemporal evolution in femtosecond second-harmonic generation with back-conversion

Jie Guo, Jianqiu Xu, Luqi Guo, Zhihua Tu et al.
Optics Express
Laser-Matter Interactions and Applications
article

Spatiotemporal evolution in femtosecond second-harmonic generation with back-conversion

Jie Guo, Jianqiu Xu, Luqi Guo, Zhihua Tu, Xiaoyan Liang, Zichen Gao, Jinfeng Li, Pukai Xue
article en

Abstract

We systematically investigate second-harmonic generation (SHG) in a lithium triborate (LBO) crystal by a femtosecond laser system (1030 nm, 195 fs, 30 W) with particular emphasis on back-conversion phenomena. For a selected 5 mm thick crystal, an optimal conversion efficiency of 54% is achieved at 18 W input power with beam quality factor M<sup>2</sup> of 1.275 (horizontal) and 1.173 (vertical). Beyond the saturation threshold where back-conversion initiates, spectral broadening, temporal compression and beam quality deterioration emerge, accompanied by decreasing conversion efficiency. Increasing the beam diameter or reducing the crystal length effectively mitigates back-conversion phenomena. These findings establish valuable guidelines for optimizing the performance of femtosecond visible laser sources.

Optics ExpressVol. 33(14)
Tongji University (CN), Chinese Academy of Sciences (CN), Shanghai Zhangjiang Laboratory (CN), University of Chinese Academy of Sciences (CN)
National Natural Science Foundation of China, Program of Shanghai Academic Research Leader
Affordable and clean energy
Openalex Percentile: Top 89%
Laser-Matter Interactions and Applications
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Spatiotemporal evolution in femtosecond second-harmonic generation with back-conversion — Jie Guo, Jianqiu Xu, et al. · Optics Express (2025) | TGRS Research Map | TGRS