C<sub>60</sub>-Supported Single Pt Atom for Selective CH<sub>4</sub> Activation
Supported single-atom catalysts (SACs) exhibit great potential for the selective activation of C-H bonds, enabling the direct conversion of methane (CH<sub>4</sub>) into high value-added chemical products. Herein, benefiting from state-of-the-art mass spectrometry coupled with newly designed variable-temperature double ion trap reactors, we successfully immobilized a single Pt<sup>-</sup> atom on a unique zero-dimensional carbon support (C<sub>60</sub>) and observed a significantly enhanced reactivity of C<sub>60</sub>Pt<sup>-</sup> toward CH<sub>4</sub> activation at room temperature compared to inert bare Pt<sup>-</sup>. The crucial role of the C<sub>60</sub> support in modifying the electronic state of the single metal site (Pt<sup>-</sup> → Pt<sup>0</sup>) was highlighted as a key factor in enhancing orbital interactions with CH<sub>4</sub>. Furthermore, the electron-buffering capability of C<sub>60</sub> also facilitates selective CH<sub>4</sub> activation by cleaving only one C-H bond. This finding not only provides atomic-scale insights into supported SACs for CH<sub>4</sub> activation but also underscores the importance of considering the positive support effects of C<sub>60</sub> in designing related catalysts for direct CH<sub>4</sub> conversion.
Authors
- Xi‐Guan Zhao
- Sheng‐Gui He (ORCID: https://orcid.org/0000-0002-9919-6909)
- H. Y. Jia (ORCID: https://orcid.org/0000-0002-1941-7119)
- Xunlei Ding (ORCID: https://orcid.org/0000-0002-9962-714X)
- B. Zang
- Jiao-Jiao Chen
- Qing‐Yu Liu (ORCID: https://orcid.org/0000-0001-9387-4310)
Institutions
- North China Electric Power University (CN)
- Chinese Academy of Sciences (CN)
- Beijing National Laboratory for Molecular Sciences (CN)
- State Key Laboratory for Structural Chemistry of Unstable and Stable Species
Publication Details
- Journal
- The Journal of Physical Chemistry Letters
- Published
- 2025-06-17
- DOI
- https://doi.org/10.1021/acs.jpclett.5c01340
- Primary Topic
- Catalytic Processes in Materials Science
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- Fundamental Research Funds for the Central Universities