Guiding Polaritonic Energy and Momentum Through 2D Bravais Lattices

Controlling polariton dispersion facilitates the study of various new physical phenomena, such as Bose-Einstein condensation, polariton lasing, and coherent quantum fluid dynamics, with manual control remaining an area of ongoing exploration. In this work, monolayer MoS<sub>2</sub> based Fabry-Pérot microcavity is used to form polaritons. Five types of Bravais lattices based on polymethyl methacrylate (PMMA) nanopillars are intentionally designed. The energy overlap between the periodic PMMA scattering wave and the polariton establishes a coupling channel that controls the directional flow of polaritonic energy, as demonstrated through angle-resolved reflectance measurements. Back-space image measurements further demonstrate that the dispersion in reciprocal space can be directly and manually tuned, allowing for control over their number and their positions. The coupling between the polariton and PMMA scattering wave is further demonstrated by analyzing the reflectance using temporal coupled-mode theory. The symmetries of 2D Bravais lattices allow the angle between energy and momentum flow to vary widely, and the position of the dispersion branch in a specific direction can be fine-tuned via lattice constant, enabling full-range control over polariton dispersion. This work presents the first theoretical and experimental demonstrations of guiding the direction of polaritonic energy and momentum through Bravais lattice design.

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Publication Details

Journal
Advanced Materials
Published
2025-06-16
DOI
https://doi.org/10.1002/adma.202505856
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
0.00

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article

Guiding Polaritonic Energy and Momentum Through 2D Bravais Lattices

Dongliang Yang, Zexiang Shen, Linfeng Sun, Wenjun Liu et al.
Advanced Materials
Strong Light-Matter Interactions
article

Guiding Polaritonic Energy and Momentum Through 2D Bravais Lattices

Dongliang Yang, Zexiang Shen, Linfeng Sun, Wenjun Liu, Zhonglin Li, Tianze Yu, Ruitong Bie, Yingying Wang
article en

Abstract

Controlling polariton dispersion facilitates the study of various new physical phenomena, such as Bose-Einstein condensation, polariton lasing, and coherent quantum fluid dynamics, with manual control remaining an area of ongoing exploration. In this work, monolayer MoS<sub>2</sub> based Fabry-Pérot microcavity is used to form polaritons. Five types of Bravais lattices based on polymethyl methacrylate (PMMA) nanopillars are intentionally designed. The energy overlap between the periodic PMMA scattering wave and the polariton establishes a coupling channel that controls the directional flow of polaritonic energy, as demonstrated through angle-resolved reflectance measurements. Back-space image measurements further demonstrate that the dispersion in reciprocal space can be directly and manually tuned, allowing for control over their number and their positions. The coupling between the polariton and PMMA scattering wave is further demonstrated by analyzing the reflectance using temporal coupled-mode theory. The symmetries of 2D Bravais lattices allow the angle between energy and momentum flow to vary widely, and the position of the dispersion branch in a specific direction can be fine-tuned via lattice constant, enabling full-range control over polariton dispersion. This work presents the first theoretical and experimental demonstrations of guiding the direction of polaritonic energy and momentum through Bravais lattice design.

Advanced MaterialsVol. 37(35)
Beijing Institute of Technology (CN), Nanyang Technological University (SG), Harbin Institute of Technology (CN)
National Natural Science Foundation of China, Natural Science Foundation of Beijing Municipality, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 89%
Strong Light-Matter Interactions
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