Dynamic Antireflection and Reflectance Terahertz Modulator via Impedance Matching Using Composite Ge<sub>2</sub>Sb<sub>2</sub>Te<sub>5</sub>/VO<sub>2</sub> Phase-Change Thin Films

Numerous functional materials have been investigated for impedance-matching-based terahertz (THz) antireflection; however, their practical utilization is significantly constrained by complex switching mechanisms, stringent excitation conditions, and challenging fabrication processes. In this study, we propose a novel method for THz wave amplitude modulation utilizing a VO<sub>2</sub>/GST(Ge<sub>2</sub>Sb<sub>2</sub>Te<sub>5</sub>) composite phase-change material interface, enabling efficient switching control and multiangle reflection modulation. By optimizing the device manufacturing process, we developed a modulation device that exhibits excellent antireflection performance at room temperature and can efficiently modulate the switching of THz signals. The unique advantages of this structure arise from the reversible phase transition properties of VO<sub>2</sub>, which enable dynamic reflection modulation. This study goes beyond temperature-driven THz modulation by exploring the potential of current-driven dynamic control, significantly enhancing the device's modulation flexibility. Experimental results show that this composite phase-change interface structure achieves an amplitude modulation depth of 89.5% and exhibits superior reflection modulation performance across a wide angular range from 15 to 45°. Notably, the proposed structure has a broad response bandwidth spanning from 0.2 to 1.5 THz, ensuring robust performance over a wide spectrum of terahertz frequencies. This innovative structure not only offers new theoretical foundations and technical pathways for designing terahertz modulation devices but also establishes a solid foundation for expanding the application domains of terahertz technology.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2025-06-16
DOI
https://doi.org/10.1021/acsami.5c07903
Citations
1
Primary Topic
Phase-change materials and chalcogenides
Type
article
Field-Weighted Citation Impact
0.52

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article

Dynamic Antireflection and Reflectance Terahertz Modulator via Impedance Matching Using Composite Ge2Sb2Te5/VO2 Phase-Change Thin Films

Xueguang Lu, Kefan Chen, Wanxia Huang, Li Chang et al.
1 citations
ACS Applied Materials & Interfaces
Phase-change materials and chalcogenides
0.52
article

Dynamic Antireflection and Reflectance Terahertz Modulator via Impedance Matching Using Composite Ge2Sb2Te5/VO2 Phase-Change Thin Films

Xueguang Lu, Kefan Chen, Wanxia Huang, Li Chang, Hongfu Zhu
article en
1 citations

Abstract

Numerous functional materials have been investigated for impedance-matching-based terahertz (THz) antireflection; however, their practical utilization is significantly constrained by complex switching mechanisms, stringent excitation conditions, and challenging fabrication processes. In this study, we propose a novel method for THz wave amplitude modulation utilizing a VO<sub>2</sub>/GST(Ge<sub>2</sub>Sb<sub>2</sub>Te<sub>5</sub>) composite phase-change material interface, enabling efficient switching control and multiangle reflection modulation. By optimizing the device manufacturing process, we developed a modulation device that exhibits excellent antireflection performance at room temperature and can efficiently modulate the switching of THz signals. The unique advantages of this structure arise from the reversible phase transition properties of VO<sub>2</sub>, which enable dynamic reflection modulation. This study goes beyond temperature-driven THz modulation by exploring the potential of current-driven dynamic control, significantly enhancing the device's modulation flexibility. Experimental results show that this composite phase-change interface structure achieves an amplitude modulation depth of 89.5% and exhibits superior reflection modulation performance across a wide angular range from 15 to 45°. Notably, the proposed structure has a broad response bandwidth spanning from 0.2 to 1.5 THz, ensuring robust performance over a wide spectrum of terahertz frequencies. This innovative structure not only offers new theoretical foundations and technical pathways for designing terahertz modulation devices but also establishes a solid foundation for expanding the application domains of terahertz technology.

ACS Applied Materials & InterfacesVol. 17(26)
Sichuan University (CN), Division of Materials Science and Engineering (AU)
National Key Research and Development Program of China
Openalex Percentile: Top 37%
Phase-change materials and chalcogenides
0.52
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