Enhancing the performance of interfacial electrocatalysts by engineering the monomer composition and sequence of metallo-oligomer monolayers
Hetero-metallo-oligomer monolayers should be superior to their monomers for interfacial electrocatalysis. Here, we present a strategy to optimize and enhance the performance of interfacial electrocatalysts by engineering the composition and sequence of distinct metal complexes. The catalytic current density of the alternating hetero-heptamer monolayers is 10 and 2.4 times higher than those of the self-assembled and homo-heptamer monolayers, respectively.
Authors
- Xuan Pang (ORCID: https://orcid.org/0000-0003-3293-832X)
- Wei Chang (ORCID: https://orcid.org/0000-0002-0222-0010)
- Lingyun Shen
- Mao Li (ORCID: https://orcid.org/0000-0003-2756-8627)
- Jing Li (ORCID: https://orcid.org/0000-0003-1811-4586)
- Yongfang Li (ORCID: https://orcid.org/0000-0002-2565-2748)
Institutions
- University of Science and Technology of China (CN)
- Jilin University (CN)
- Chinese Academy of Sciences (CN)
- Changchun Institute of Applied Chemistry (CN)
- State Key Laboratory of Polymer Physics and Chemistry (CN)
- State Key Laboratory of Supramolecular Structure and Materials
Publication Details
- Journal
- Chemical Communications
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5cc02175h
- Primary Topic
- Fuel Cells and Related Materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00