Field-resolved attosecond solitons

Abstract Here we harness soliton dynamics in a hollow-core fibre to generate attosecond laser pulses spanning the deep ultraviolet (DUV) to the near infrared, and we record their electric-field waveforms using nonlinear photoconductive sampling. By combining these techniques, we measure ultrashort pulses containing a soliton at optical wavelengths and generated a resonant dispersive wave covering the DUV regime with a total pulse duration of 350 attoseconds full width at half maximum of the squared field, demonstrating the extension of the electric-field sampling bandwidth to ultrashort wavelengths. Therefore, we provide a flexible and efficient route to the generation of intense isolated attosecond pulses complementary to those based on high-harmonic generation in gases, in a spectral range particularly interesting for studies in solids and in molecules. Finally, we show that these subcycle DUV–near-infrared pulses provide sufficient intensities to ionize argon and, thus, access attosecond strong-field laser physics in these spectral regions.

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Publication Details

Journal
Nature Photonics
Published
2025-06-13
DOI
https://doi.org/10.1038/s41566-025-01658-5
Citations
15
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
18.70

Funders

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article

Field-resolved attosecond solitons

Francesco Tani, Amelie M. Heinzerling, Ferenc Krausz, Nicholas Karpowicz et al.
15 citations
Nature Photonics
Laser-Matter Interactions and Applications
18.70
article

Field-resolved attosecond solitons

Francesco Tani, Amelie M. Heinzerling, Ferenc Krausz, Nicholas Karpowicz, Vladislav S. Yakovlev, Manoram Agarwal
article en
15 citations

Abstract

Abstract Here we harness soliton dynamics in a hollow-core fibre to generate attosecond laser pulses spanning the deep ultraviolet (DUV) to the near infrared, and we record their electric-field waveforms using nonlinear photoconductive sampling. By combining these techniques, we measure ultrashort pulses containing a soliton at optical wavelengths and generated a resonant dispersive wave covering the DUV regime with a total pulse duration of 350 attoseconds full width at half maximum of the squared field, demonstrating the extension of the electric-field sampling bandwidth to ultrashort wavelengths. Therefore, we provide a flexible and efficient route to the generation of intense isolated attosecond pulses complementary to those based on high-harmonic generation in gases, in a spectral range particularly interesting for studies in solids and in molecules. Finally, we show that these subcycle DUV–near-infrared pulses provide sufficient intensities to ionize argon and, thus, access attosecond strong-field laser physics in these spectral regions.

Nature PhotonicsVol. 19(7)
Centre National de la Recherche Scientifique (FR), Université de Lille (FR), Max Planck Institute for the Science of Light (DE), Max Planck Institute of Quantum Optics (DE), Laboratoire de Physique des Lasers, Atomes et Molécules (FR), Ludwig-Maximilians-Universität München (DE)
International Max Planck Research School for Environmental, Cellular and Molecular Microbiology, Max-Planck-Gesellschaft, International Max Planck Research School for Advanced Methods in Process and Systems Engineering
Openalex Percentile: Top 1%
Laser-Matter Interactions and Applications
18.70
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