Engineered chirality of one-dimensional nanowires

The origin and function of chirality in DNA, proteins, and other building blocks of life represent a central question in biology. Observations of spin polarization and magnetization associated with electron transport through chiral molecules, known collectively as the chiral induced spin selectivity effect, suggest that chirality improves electron transfer. Using reconfigurable nanoscale control over conductivity at the LaAlO<sub>3</sub>/SrTiO<sub>3</sub> interface, we create chiral electron potentials that explicitly lack mirror symmetry. Quantum transport measurements on these chiral nanowires reveal enhanced electron pairing persisting to high magnetic fields (up to 18 tesla) and oscillatory transmission resonances as functions of both magnetic field and chemical potential. We interpret these resonances as arising from an engineered axial spin-orbit interaction within the chiral region. The ability to create one-dimensional electron waveguides with this specificity creates opportunities to test, via analog quantum simulation, theories about chirality and spin-polarized electron transport in one-dimensional geometries.

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Publication Details

Journal
Science Advances
Published
2025-06-13
DOI
https://doi.org/10.1126/sciadv.adx4761
Citations
4
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
2.07
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article

Engineered chirality of one-dimensional nanowires

Megan Briggeman, Elliott Mansfield, Andrew J. Daley, Johannes Kombe et al.
4 citations
Science Advances
Electronic and Structural Properties of Oxides
2.07
article

Engineered chirality of one-dimensional nanowires

Megan Briggeman, Elliott Mansfield, Andrew J. Daley, Johannes Kombe, Mengchen Huang, Jeremy Levy, Muqing Yu, François Damanet, Patrick Irvin, Chang‐Beom Eom, Jianan Li, Hyungwoo Lee, Sayanwita Biswas, Yuhe Tang
article en
4 citations

Abstract

The origin and function of chirality in DNA, proteins, and other building blocks of life represent a central question in biology. Observations of spin polarization and magnetization associated with electron transport through chiral molecules, known collectively as the chiral induced spin selectivity effect, suggest that chirality improves electron transfer. Using reconfigurable nanoscale control over conductivity at the LaAlO<sub>3</sub>/SrTiO<sub>3</sub> interface, we create chiral electron potentials that explicitly lack mirror symmetry. Quantum transport measurements on these chiral nanowires reveal enhanced electron pairing persisting to high magnetic fields (up to 18 tesla) and oscillatory transmission resonances as functions of both magnetic field and chemical potential. We interpret these resonances as arising from an engineered axial spin-orbit interaction within the chiral region. The ability to create one-dimensional electron waveguides with this specificity creates opportunities to test, via analog quantum simulation, theories about chirality and spin-polarized electron transport in one-dimensional geometries.

Science AdvancesVol. 11(24)
University of Wisconsin–Madison (US), University of Liège (BE), University of Pittsburgh (US), University of Strathclyde (GB), University of Oxford (GB), Pittsburgh Quantum Institute (US)
Openalex Percentile: Top 13%
Electronic and Structural Properties of Oxides
2.07
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