Tunable orbital thermoelectric transport with spin-valley coupling in a monolayer of ferromagnetic transition metal dichalcogenides

The valley transport of electrons can carry not only charge but also spin angular momentum and orbital angular momentum (OAM). However, investigations on thermoelectric transport of OAM manipulated by valley degrees of freedom remain limited. Here, using the ferromagnetic transition metal dichalcogenides ${\mathrm{RuCl}}_{2}$ as an example, we investigate valley-contrasting Berry curvature and demonstrate its role in generating valley-dependent anomalous and orbital Nernst effects. The thermoelectric transport of OAM is shown to be modulated by intrinsic spin polarization and exhibits characteristics of valley-orbital coupling. Furthermore, we show that spin-valley coupling plays a crucial role in controlling the orbital Nernst effect and distinguishing it from the anomalous Nernst effect. Based on these findings, we propose a thermoelectric transport mechanism for generating pure orbital currents.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-06-09
DOI
https://doi.org/10.1103/physrevb.111.235417
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Tunable orbital thermoelectric transport with spin-valley coupling in a monolayer of ferromagnetic transition metal dichalcogenides

Jianping Yang, Li Hua Gao, Shilei Ji, Xing’ao Li
Physical review. B./Physical review. B
2D Materials and Applications
article

Tunable orbital thermoelectric transport with spin-valley coupling in a monolayer of ferromagnetic transition metal dichalcogenides

Jianping Yang, Li Hua Gao, Shilei Ji, Xing’ao Li
article en

Abstract

The valley transport of electrons can carry not only charge but also spin angular momentum and orbital angular momentum (OAM). However, investigations on thermoelectric transport of OAM manipulated by valley degrees of freedom remain limited. Here, using the ferromagnetic transition metal dichalcogenides ${\mathrm{RuCl}}_{2}$ as an example, we investigate valley-contrasting Berry curvature and demonstrate its role in generating valley-dependent anomalous and orbital Nernst effects. The thermoelectric transport of OAM is shown to be modulated by intrinsic spin polarization and exhibits characteristics of valley-orbital coupling. Furthermore, we show that spin-valley coupling plays a crucial role in controlling the orbital Nernst effect and distinguishing it from the anomalous Nernst effect. Based on these findings, we propose a thermoelectric transport mechanism for generating pure orbital currents.

Physical review. B./Physical review. BVol. 111(23)
Nanjing University of Posts and Telecommunications (CN)
National Natural Science Foundation of China, Nanjing University of Posts and Telecommunications, Jiangsu Provincial Key Research and Development Program
Openalex Percentile: Top 91%
2D Materials and Applications
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Tunable orbital thermoelectric transport with spin-valley coupling in a monolayer of ferromagnetic transition metal dichalcogenides — Jianping Yang, Li Hua Gao, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS