Band structure reconstruction in the topological semimetal PrAlSi

The interplay between nontrivial topology, magnetism, and strong correlation has generated considerable research interest in condensed matter physics. The topological $R\text{Al}X$ ($R$ = rare earth; $X$ = Si and Ge) family has provided an excellent platform for exploring these complex interactions. Here, we performed infrared spectroscopy measurements on the ferromagnetic (FM) topological semimetal PrAlSi, in order to investigate the impact of FM orderings on the topological band structure. We find that the optical conductivity associated with the Dirac/Weyl cones exhibits two segments of linearly increasing parts in the normal state, connected by a kink feature at around 1960 ${\mathrm{cm}}^{\ensuremath{-}1}$. By entering the FM state, however, an additional linear-growing segment shows up in between the original ones, suggesting that the band structure is reconstructed. We propose that these observations can be effectively explained by a scenario where the Dirac/Weyl nodes are split into pairs of Weyl nodes with lower degeneracy, due to the time reversal symmetry breaking induced by the FM ordering. This band structure reconstruction also leads to a sudden enhancement of the itinerant carrier density. In addition, the effective mass of the itinerant carriers are estimated to be three orders of magnitude smaller than the free electron mass, providing a rare case where nearly all the free carriers exhibit behaviors characteristic of relativistic Dirac or Weyl fermions. Our results demonstrate a compelling example of the strong interaction between magnetic order and topological band structures, which opens up new avenues for exploring novel topological materials and their potential applications.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-06-09
DOI
https://doi.org/10.1103/physrevb.111.245125
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Band structure reconstruction in the topological semimetal PrAlSi

Peijie Sun, Bin Gao, X. Y. Zhang, Ming‐Ju Amy Lyu et al.
Physical review. B./Physical review. B
Topological Materials and Phenomena
article

Band structure reconstruction in the topological semimetal PrAlSi

Peijie Sun, Bin Gao, X. Y. Zhang, Ming‐Ju Amy Lyu, X. T. Zhang, L. Y. Cao, Lirong Wang, R. Y. Chen
article en

Abstract

The interplay between nontrivial topology, magnetism, and strong correlation has generated considerable research interest in condensed matter physics. The topological $R\text{Al}X$ ($R$ = rare earth; $X$ = Si and Ge) family has provided an excellent platform for exploring these complex interactions. Here, we performed infrared spectroscopy measurements on the ferromagnetic (FM) topological semimetal PrAlSi, in order to investigate the impact of FM orderings on the topological band structure. We find that the optical conductivity associated with the Dirac/Weyl cones exhibits two segments of linearly increasing parts in the normal state, connected by a kink feature at around 1960 ${\mathrm{cm}}^{\ensuremath{-}1}$. By entering the FM state, however, an additional linear-growing segment shows up in between the original ones, suggesting that the band structure is reconstructed. We propose that these observations can be effectively explained by a scenario where the Dirac/Weyl nodes are split into pairs of Weyl nodes with lower degeneracy, due to the time reversal symmetry breaking induced by the FM ordering. This band structure reconstruction also leads to a sudden enhancement of the itinerant carrier density. In addition, the effective mass of the itinerant carriers are estimated to be three orders of magnitude smaller than the free electron mass, providing a rare case where nearly all the free carriers exhibit behaviors characteristic of relativistic Dirac or Weyl fermions. Our results demonstrate a compelling example of the strong interaction between magnetic order and topological band structures, which opens up new avenues for exploring novel topological materials and their potential applications.

Physical review. B./Physical review. BVol. 111(24)
Chinese Academy of Sciences (CN), Beijing Normal University (CN), Songshan Lake Materials Laboratory (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Institute of Physics (CN), University of Chinese Academy of Sciences (CN)
National Natural Science Foundation of China, Natural Science Foundation for Young Scientists of Shanxi Province, National Key Research and Development Program of China, Fundamental Research Funds for the Central Universities
Sustainable cities and communities
Openalex Percentile: Top 90%
Topological Materials and Phenomena
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