Polaron–Polariton Bose–Einstein Condensation Lasing via Longitudinal Optical Phonon Scattering in GaN-Based Microcavity

Exciton-polaritons, hybrid states composed of excitons and photons under strong coupling, play a crucial role in investigating Bose-Einstein condensation (BEC) and optoelectronics. However, the relaxation bottleneck in exciton-polaritons, arising from reduced scattering efficiency with acoustic phonons, hinders the achievement of thermal equilibrium Bose-Einstein condensation (BEC). Here, by invoking the polaronic effect of the exciton, we present the first observation of polaron-polariton BEC in a GaN-based microcavity. The dispersion pattern in k-space reveals a typical middle polariton (MP) branch of polaron-polaritons. This unique dispersion structure enables a novel relaxation route through LO-phonon-mediated scattering for polaron-polaritons, overcoming the phonon bottleneck observed in exciton-polaritons. By utilizing this mechanism, we achieve a robust polaron-polariton BEC, which is confirmed by the characteristics of massive occupation of the ground state, linear polarization buildup, and long-range spatial coherence. Our findings provide new insights into thermal equilibrium BEC and high-performance polariton quantum devices with GaN materials.

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Publication Details

Journal
Nano Letters
Published
2025-06-09
DOI
https://doi.org/10.1021/acs.nanolett.5c01198
Citations
2
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
2.49

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article

Polaron–Polariton Bose–Einstein Condensation Lasing via Longitudinal Optical Phonon Scattering in GaN-Based Microcavity

Jingzhuo Wang, Yiyun Zhang, Hai Zhu, Xuebing Gong et al.
2 citations
Nano Letters
Strong Light-Matter Interactions
2.49
article

Polaron–Polariton Bose–Einstein Condensation Lasing via Longitudinal Optical Phonon Scattering in GaN-Based Microcavity

Jingzhuo Wang, Yiyun Zhang, Hai Zhu, Xuebing Gong, Huying Zheng, Yifan Zhang, Shi Hua, Xianghu Wang, Runchen Wang, Dezhen Shen, Junxing Dong, Lisheng Wang
article en
2 citations

Abstract

Exciton-polaritons, hybrid states composed of excitons and photons under strong coupling, play a crucial role in investigating Bose-Einstein condensation (BEC) and optoelectronics. However, the relaxation bottleneck in exciton-polaritons, arising from reduced scattering efficiency with acoustic phonons, hinders the achievement of thermal equilibrium Bose-Einstein condensation (BEC). Here, by invoking the polaronic effect of the exciton, we present the first observation of polaron-polariton BEC in a GaN-based microcavity. The dispersion pattern in k-space reveals a typical middle polariton (MP) branch of polaron-polaritons. This unique dispersion structure enables a novel relaxation route through LO-phonon-mediated scattering for polaron-polaritons, overcoming the phonon bottleneck observed in exciton-polaritons. By utilizing this mechanism, we achieve a robust polaron-polariton BEC, which is confirmed by the characteristics of massive occupation of the ground state, linear polarization buildup, and long-range spatial coherence. Our findings provide new insights into thermal equilibrium BEC and high-performance polariton quantum devices with GaN materials.

Nano LettersVol. 25(24)
Sun Yat-sen University (CN), Chinese Academy of Sciences (CN), Suzhou Research Institute (CN), Institute of Semiconductors (CN), Shanghai Dianji University (CN), University of Chinese Academy of Sciences (CN), T.K.M. College of Arts and Science, State Key Laboratory of Optoelectronic Materials and Technology
National Natural Science Foundation of China, Fundamental Research Funds for the Central Universities
Affordable and clean energy
Openalex Percentile: Top 11%
Strong Light-Matter Interactions
2.49
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