Polaron–Polariton Bose–Einstein Condensation Lasing via Longitudinal Optical Phonon Scattering in GaN-Based Microcavity
Exciton-polaritons, hybrid states composed of excitons and photons under strong coupling, play a crucial role in investigating Bose-Einstein condensation (BEC) and optoelectronics. However, the relaxation bottleneck in exciton-polaritons, arising from reduced scattering efficiency with acoustic phonons, hinders the achievement of thermal equilibrium Bose-Einstein condensation (BEC). Here, by invoking the polaronic effect of the exciton, we present the first observation of polaron-polariton BEC in a GaN-based microcavity. The dispersion pattern in k-space reveals a typical middle polariton (MP) branch of polaron-polaritons. This unique dispersion structure enables a novel relaxation route through LO-phonon-mediated scattering for polaron-polaritons, overcoming the phonon bottleneck observed in exciton-polaritons. By utilizing this mechanism, we achieve a robust polaron-polariton BEC, which is confirmed by the characteristics of massive occupation of the ground state, linear polarization buildup, and long-range spatial coherence. Our findings provide new insights into thermal equilibrium BEC and high-performance polariton quantum devices with GaN materials.
Authors
- Jingzhuo Wang (ORCID: https://orcid.org/0000-0001-5276-4588)
- Yiyun Zhang (ORCID: https://orcid.org/0000-0002-1419-485X)
- Hai Zhu (ORCID: https://orcid.org/0000-0003-2874-5509)
- Xuebing Gong
- Huying Zheng
- Yifan Zhang (ORCID: https://orcid.org/0000-0003-1298-5436)
- Shi Hua (ORCID: https://orcid.org/0009-0003-6043-2788)
- Xianghu Wang (ORCID: https://orcid.org/0000-0002-7556-1051)
- Runchen Wang (ORCID: https://orcid.org/0000-0003-1969-7859)
- Dezhen Shen
- Junxing Dong
- Lisheng Wang (ORCID: https://orcid.org/0009-0003-6836-6156)
Institutions
- Sun Yat-sen University (CN)
- Chinese Academy of Sciences (CN)
- Suzhou Research Institute (CN)
- Institute of Semiconductors (CN)
- Shanghai Dianji University (CN)
- University of Chinese Academy of Sciences (CN)
- T.K.M. College of Arts and Science
- State Key Laboratory of Optoelectronic Materials and Technology
Publication Details
- Journal
- Nano Letters
- Published
- 2025-06-09
- DOI
- https://doi.org/10.1021/acs.nanolett.5c01198
- Citations
- 2
- Primary Topic
- Strong Light-Matter Interactions
- Type
- article
- Field-Weighted Citation Impact
- 2.49
Funders
- National Natural Science Foundation of China
- Fundamental Research Funds for the Central Universities