Oscillate and renormalize: Fast phonons reshape the Kondo effect in flat-band systems

We examine the interplay between electron correlations and phonons in an Anderson-Holstein impurity model with an Einstein phonon. When the phonons are slow compared to charge fluctuations (frequency $ω_0 \ll U/2$, the onsite Coulomb scale $U/2$), we demonstrate analytically that the expected phonon-mediated reduction of interactions is completely suppressed, even in the strong coupling regime. This suppression arises from the oscillator's inability to respond to rapid charge fluctuations, manifested as a compensation effect between the polaronic cloud and the excited-state phonons associated with valence fluctuations. We identify a novel frozen mixed valence phase, above a threshold dimensionless electron-phonon coupling $α^*$ when the phonons are slow, where the static phonon cloud locks the impurity into specific valence configurations, potentially explaining the puzzling coexistence of mixed valence behavior and insulating properties in materials like rust. Conversely, when the phonon is fast ($ω_0 \gtrsim U/2$), the system exhibits conventional polaronic behavior with renormalized onsite interactions effectively $U_{\text{eff}}$ due to phonon mediated attraction, with additional satellite features in the local spectral function due to phonon excitations. Using numerical renormalization group (NRG) calculations, a fully dynamic renormalization technique, we confirm these behaviors in both regimes. These findings have important implications for strongly correlated systems where phonon energy scales may be comparable to the Coulomb scale, such as in twisted bilayer graphene, necessitating careful consideration of interaction renormalizations in theoretical models.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-06-03
DOI
https://doi.org/10.1103/xxyt-4bql
Citations
1
Primary Topic
Thermal properties of materials
Type
article
Field-Weighted Citation Impact
0.52
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article

Oscillate and renormalize: Fast phonons reshape the Kondo effect in flat-band systems

Daniel Kaplan, Piers Coleman, Andreas Gleis, Premala Chandra et al.
1 citations
Physical review. B./Physical review. B
Thermal properties of materials
0.52
article

Oscillate and renormalize: Fast phonons reshape the Kondo effect in flat-band systems

Daniel Kaplan, Piers Coleman, Andreas Gleis, Premala Chandra, Karl J. Friston
article en
1 citations

Abstract

We examine the interplay between electron correlations and phonons in an Anderson-Holstein impurity model with an Einstein phonon. When the phonons are slow compared to charge fluctuations (frequency $ω_0 \ll U/2$, the onsite Coulomb scale $U/2$), we demonstrate analytically that the expected phonon-mediated reduction of interactions is completely suppressed, even in the strong coupling regime. This suppression arises from the oscillator's inability to respond to rapid charge fluctuations, manifested as a compensation effect between the polaronic cloud and the excited-state phonons associated with valence fluctuations. We identify a novel frozen mixed valence phase, above a threshold dimensionless electron-phonon coupling $α^*$ when the phonons are slow, where the static phonon cloud locks the impurity into specific valence configurations, potentially explaining the puzzling coexistence of mixed valence behavior and insulating properties in materials like rust. Conversely, when the phonon is fast ($ω_0 \gtrsim U/2$), the system exhibits conventional polaronic behavior with renormalized onsite interactions effectively $U_{\text{eff}}$ due to phonon mediated attraction, with additional satellite features in the local spectral function due to phonon excitations. Using numerical renormalization group (NRG) calculations, a fully dynamic renormalization technique, we confirm these behaviors in both regimes. These findings have important implications for strongly correlated systems where phonon energy scales may be comparable to the Coulomb scale, such as in twisted bilayer graphene, necessitating careful consideration of interaction renormalizations in theoretical models.

Physical review. B./Physical review. BVol. 111(24)
Rutgers, The State University of New Jersey (US), Rutgers Sexual and Reproductive Health and Rights (NL)
Openalex Percentile: Top 38%
Thermal properties of materials
0.52
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