Perfecting Phase Matching in Nonlinear Resonant Photonic Structures via Green’s Function Integral Formalism

Phase mismatch poses a key challenge in nonlinear photonics, where existing methods generally fail to characterize the localized phase mismatch. Here, we demonstrate the Green’s function integral method (GFIM) as a fundamental analytical framework for microscopic phase engineering, enabling perfect phase matching in χ(2)-based resonant structures. By modeling second-harmonic generation as the integration (or superposition) of subharmonic components generated by microscopic nonlinear sources, GFIM permits precise identification of phase mismatch at the microscopic scale and establishes a quantitative metric for assessing phase-matching efficiency. Our phase analysis reveals that the triple-DBR resonator induces periodic π-phase discontinuities of subharmonic fields, allowing for a refined quasi-phase matching technique that converts destructive-to-constructive interference, thereby achieving unprecedented perfect phase matching. In a 2 μm nonlinear film, this approach yields a calculated 14% harmonic efficiency under 1 MW/cm2 pumping. With its capability to decode complicated phase distributions, GFIM emerges as an essential framework for the microscopic phase analysis and rational optimization of nonlinear photonic devices.

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Publication Details

Journal
ACS Photonics
Published
2025-06-02
DOI
https://doi.org/10.1021/acsphotonics.5c00776
Primary Topic
Photonic and Optical Devices
Type
article
Field-Weighted Citation Impact
0.00

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article

Perfecting Phase Matching in Nonlinear Resonant Photonic Structures via Green’s Function Integral Formalism

Hao Zheng, Junbing Zhou, Pingqi Gao, Chengkang Liang et al.
ACS Photonics
Photonic and Optical Devices
article

Perfecting Phase Matching in Nonlinear Resonant Photonic Structures via Green’s Function Integral Formalism

Hao Zheng, Junbing Zhou, Pingqi Gao, Chengkang Liang, Jiancan Yu
article en

Abstract

Phase mismatch poses a key challenge in nonlinear photonics, where existing methods generally fail to characterize the localized phase mismatch. Here, we demonstrate the Green’s function integral method (GFIM) as a fundamental analytical framework for microscopic phase engineering, enabling perfect phase matching in χ(2)-based resonant structures. By modeling second-harmonic generation as the integration (or superposition) of subharmonic components generated by microscopic nonlinear sources, GFIM permits precise identification of phase mismatch at the microscopic scale and establishes a quantitative metric for assessing phase-matching efficiency. Our phase analysis reveals that the triple-DBR resonator induces periodic π-phase discontinuities of subharmonic fields, allowing for a refined quasi-phase matching technique that converts destructive-to-constructive interference, thereby achieving unprecedented perfect phase matching. In a 2 μm nonlinear film, this approach yields a calculated 14% harmonic efficiency under 1 MW/cm2 pumping. With its capability to decode complicated phase distributions, GFIM emerges as an essential framework for the microscopic phase analysis and rational optimization of nonlinear photonic devices.

ACS PhotonicsVol. 12(6)
Sun Yat-sen University (CN)
National Natural Science Foundation of China
Openalex Percentile: Top 90%
Photonic and Optical Devices
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Perfecting Phase Matching in Nonlinear Resonant Photonic Structures via Green’s Function Integral Formalism — Hao Zheng, Junbing Zhou, et al. · ACS Photonics (2025) | TGRS Research Map | TGRS