Quantum emitter in a plasmonic field: An orientation-generalized model

When a quantum emitter (QE) is placed in close proximity to a plasmonic metal nanoparticle within an external optical field, a dipole-dipole coupling arises, resulting in a highly tunable hybrid nanosystem that surpasses the optical manipulation capabilities of the individual components. These hybrid systems enable the exploration and manipulation of optical fields at the intersection between classical and quantum phenomena. Theoretical models of this interaction have typically been limited to the extreme orientations, where the QE and plasmonic dipoles are polarized either along or perpendicular to the interparticle axis, for analytical tractability. In this work, we generalize the semiclassical optical dipole-dipole interaction model for a two-level quantum emitter in a plasmonic field for arbitrary polarization angles. We show that the total field experienced by the quantum emitter at intermediate angles does not necessarily align with the external input field and discuss the implications of varying the polarization angle of the external input field.

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Publication Details

Journal
Physical Review Research
Published
2025-05-30
DOI
https://doi.org/10.1103/physrevresearch.7.023206
Citations
1
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
0.67

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article

Quantum emitter in a plasmonic field: An orientation-generalized model

Jared H. Cole, Harini Hapuarachchi, Jesse A. Vaitkus
1 citations
Physical Review Research
Plasmonic and Surface Plasmon Research
0.67
article

Quantum emitter in a plasmonic field: An orientation-generalized model

Jared H. Cole, Harini Hapuarachchi, Jesse A. Vaitkus
article en
1 citations

Abstract

When a quantum emitter (QE) is placed in close proximity to a plasmonic metal nanoparticle within an external optical field, a dipole-dipole coupling arises, resulting in a highly tunable hybrid nanosystem that surpasses the optical manipulation capabilities of the individual components. These hybrid systems enable the exploration and manipulation of optical fields at the intersection between classical and quantum phenomena. Theoretical models of this interaction have typically been limited to the extreme orientations, where the QE and plasmonic dipoles are polarized either along or perpendicular to the interparticle axis, for analytical tractability. In this work, we generalize the semiclassical optical dipole-dipole interaction model for a two-level quantum emitter in a plasmonic field for arbitrary polarization angles. We show that the total field experienced by the quantum emitter at intermediate angles does not necessarily align with the external input field and discuss the implications of varying the polarization angle of the external input field.

Physical Review ResearchVol. 7(2)
MIT University (MK), RMIT University (AU)
National Computational Infrastructure, Australian Government, RMIT University, Australian Research Council, National Cancer Institute, Centre of Excellence in Exciton Science
Openalex Percentile: Top 31%
Plasmonic and Surface Plasmon Research
0.67
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