Incommensurate Antiferromagnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> under Pressure
The discovery of multiple superconducting phases in <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>UTe</a:mi></a:mrow><a:mrow><a:mn>2</a:mn></a:mrow></a:msub></a:mrow></a:math> boosted research on correlated-electron physics. This heavy-fermion paramagnet was rapidly identified as a reference compound to study the interplay between magnetism and unconventional superconductivity with multiple degrees of freedom. The proximity to a ferromagnetic quantum phase transition was initially proposed as a driving force to triplet-pairing superconductivity. However, we find here that long-range incommensurate antiferromagnetic order is established under pressure. The propagation vector <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:msub><c:mi mathvariant="bold">k</c:mi><c:mi mathvariant="bold">m</c:mi></c:msub><c:mo>=</c:mo><c:mo stretchy="false">(</c:mo><c:mn>0.07</c:mn><c:mo>,</c:mo><c:mn>0.33</c:mn><c:mo>,</c:mo><c:mn>1</c:mn><c:mo stretchy="false">)</c:mo></c:math> of the antiferromagnetic phase is close to a wave vector where antiferromagnetic fluctuations have previously been observed at ambient pressure. These elements support that <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:mrow><i:msub><i:mrow><i:mi>UTe</i:mi></i:mrow><i:mrow><i:mn>2</i:mn></i:mrow></i:msub></i:mrow></i:math> is a nearly antiferromagnet at ambient pressure. Our work appeals for theories modeling the evolution of the magnetic interactions and electronic properties, driving a correlated paramagnetic regime at ambient pressure to a long-range antiferromagnetic order under pressure. A deeper understanding of itinerant-<k:math xmlns:k="http://www.w3.org/1998/Math/MathML" display="inline"><k:mi>f</k:mi></k:math>-electron magnetism in <m:math xmlns:m="http://www.w3.org/1998/Math/MathML" display="inline"><m:mrow><m:msub><m:mrow><m:mi>UTe</m:mi></m:mrow><m:mrow><m:mn>2</m:mn></m:mrow></m:msub></m:mrow></m:math> will be a key for describing its unconventional superconducting phases.
Authors
- S. Raymond (ORCID: https://orcid.org/0000-0002-5421-5061)
- Dai Aoki (ORCID: https://orcid.org/0000-0003-2334-8360)
- T. Thebault (ORCID: https://orcid.org/0000-0002-3034-4838)
- G. Knebel (ORCID: https://orcid.org/0000-0002-0442-6362)
- D. D. Khalyavin (ORCID: https://orcid.org/0000-0002-6724-7695)
- Koji Kaneko (ORCID: https://orcid.org/0000-0002-2002-0610)
- W. Knafo (ORCID: https://orcid.org/0000-0001-7100-9166)
- G. Lapertot (ORCID: https://orcid.org/0000-0001-6023-478X)
- E. Ressouche (ORCID: https://orcid.org/0000-0001-6364-1890)
- D. Braithwaite (ORCID: https://orcid.org/0000-0002-9012-4255)
- K. Beauvois (ORCID: https://orcid.org/0009-0001-6137-1644)
- Fabio Orlandi (ORCID: https://orcid.org/0000-0001-6333-521X)
- Pascal Manuel (ORCID: https://orcid.org/0000-0002-8845-6576)
Institutions
- Institut polytechnique de Grenoble (FR)
- Japan Atomic Energy Agency (JP)
- Rutherford Appleton Laboratory (GB)
- Tohoku University (JP)
- Commissariat à l'Énergie Atomique et aux Énergies Alternatives (FR)
- CEA Grenoble (FR)
- Laboratoire National des Champs Magnétiques Intenses (FR)
- China Spallation Neutron Source (CN)
- Advanced Science Research Center (JP)
- ISIS Neutron and Muon Source
- Université Grenoble Alpes (FR)
Publication Details
- Journal
- Physical Review X
- Published
- 2025-05-30
- DOI
- https://doi.org/10.1103/physrevx.15.021075
- Citations
- 4
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 5.03
Funders
- Agence Nationale de la Recherche
- Japan Society for the Promotion of Science