Incommensurate Antiferromagnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> under Pressure

The discovery of multiple superconducting phases in <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>UTe</a:mi></a:mrow><a:mrow><a:mn>2</a:mn></a:mrow></a:msub></a:mrow></a:math> boosted research on correlated-electron physics. This heavy-fermion paramagnet was rapidly identified as a reference compound to study the interplay between magnetism and unconventional superconductivity with multiple degrees of freedom. The proximity to a ferromagnetic quantum phase transition was initially proposed as a driving force to triplet-pairing superconductivity. However, we find here that long-range incommensurate antiferromagnetic order is established under pressure. The propagation vector <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:msub><c:mi mathvariant="bold">k</c:mi><c:mi mathvariant="bold">m</c:mi></c:msub><c:mo>=</c:mo><c:mo stretchy="false">(</c:mo><c:mn>0.07</c:mn><c:mo>,</c:mo><c:mn>0.33</c:mn><c:mo>,</c:mo><c:mn>1</c:mn><c:mo stretchy="false">)</c:mo></c:math> of the antiferromagnetic phase is close to a wave vector where antiferromagnetic fluctuations have previously been observed at ambient pressure. These elements support that <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:mrow><i:msub><i:mrow><i:mi>UTe</i:mi></i:mrow><i:mrow><i:mn>2</i:mn></i:mrow></i:msub></i:mrow></i:math> is a nearly antiferromagnet at ambient pressure. Our work appeals for theories modeling the evolution of the magnetic interactions and electronic properties, driving a correlated paramagnetic regime at ambient pressure to a long-range antiferromagnetic order under pressure. A deeper understanding of itinerant-<k:math xmlns:k="http://www.w3.org/1998/Math/MathML" display="inline"><k:mi>f</k:mi></k:math>-electron magnetism in <m:math xmlns:m="http://www.w3.org/1998/Math/MathML" display="inline"><m:mrow><m:msub><m:mrow><m:mi>UTe</m:mi></m:mrow><m:mrow><m:mn>2</m:mn></m:mrow></m:msub></m:mrow></m:math> will be a key for describing its unconventional superconducting phases.

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Institutions

Publication Details

Journal
Physical Review X
Published
2025-05-30
DOI
https://doi.org/10.1103/physrevx.15.021075
Citations
4
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
5.03

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article

Incommensurate Antiferromagnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> under Pressure

S. Raymond, Dai Aoki, T. Thebault, G. Knebel et al.
4 citations
Physical Review X
Rare-earth and actinide compounds
5.03
article

Incommensurate Antiferromagnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> under Pressure

S. Raymond, Dai Aoki, T. Thebault, G. Knebel, D. D. Khalyavin, Koji Kaneko, W. Knafo, G. Lapertot, E. Ressouche, D. Braithwaite, K. Beauvois, Fabio Orlandi, Pascal Manuel
article en
4 citations

Abstract

The discovery of multiple superconducting phases in <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>UTe</a:mi></a:mrow><a:mrow><a:mn>2</a:mn></a:mrow></a:msub></a:mrow></a:math> boosted research on correlated-electron physics. This heavy-fermion paramagnet was rapidly identified as a reference compound to study the interplay between magnetism and unconventional superconductivity with multiple degrees of freedom. The proximity to a ferromagnetic quantum phase transition was initially proposed as a driving force to triplet-pairing superconductivity. However, we find here that long-range incommensurate antiferromagnetic order is established under pressure. The propagation vector <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:msub><c:mi mathvariant="bold">k</c:mi><c:mi mathvariant="bold">m</c:mi></c:msub><c:mo>=</c:mo><c:mo stretchy="false">(</c:mo><c:mn>0.07</c:mn><c:mo>,</c:mo><c:mn>0.33</c:mn><c:mo>,</c:mo><c:mn>1</c:mn><c:mo stretchy="false">)</c:mo></c:math> of the antiferromagnetic phase is close to a wave vector where antiferromagnetic fluctuations have previously been observed at ambient pressure. These elements support that <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:mrow><i:msub><i:mrow><i:mi>UTe</i:mi></i:mrow><i:mrow><i:mn>2</i:mn></i:mrow></i:msub></i:mrow></i:math> is a nearly antiferromagnet at ambient pressure. Our work appeals for theories modeling the evolution of the magnetic interactions and electronic properties, driving a correlated paramagnetic regime at ambient pressure to a long-range antiferromagnetic order under pressure. A deeper understanding of itinerant-<k:math xmlns:k="http://www.w3.org/1998/Math/MathML" display="inline"><k:mi>f</k:mi></k:math>-electron magnetism in <m:math xmlns:m="http://www.w3.org/1998/Math/MathML" display="inline"><m:mrow><m:msub><m:mrow><m:mi>UTe</m:mi></m:mrow><m:mrow><m:mn>2</m:mn></m:mrow></m:msub></m:mrow></m:math> will be a key for describing its unconventional superconducting phases.

Physical Review XVol. 15(2)
Institut polytechnique de Grenoble (FR), Japan Atomic Energy Agency (JP), Rutherford Appleton Laboratory (GB), Tohoku University (JP), Commissariat à l'Énergie Atomique et aux Énergies Alternatives (FR), CEA Grenoble (FR), Laboratoire National des Champs Magnétiques Intenses (FR), China Spallation Neutron Source (CN), Advanced Science Research Center (JP), ISIS Neutron and Muon Source, Université Grenoble Alpes (FR)
Agence Nationale de la Recherche, Japan Society for the Promotion of Science
Openalex Percentile: Top 5%
Rare-earth and actinide compounds
5.03
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