Quasi-Ballistic Heat Conduction of Long-Range Surface Phonon Polaritons Coupled to Thermal Reservoirs

Rigorous thermal control at the nanoscale has become essential with the miniaturization of electronic devices. However, heat transfer in such structures is hindered by increased boundary scatterings and reduced thermal conductivity. Surface phonon polaritons (SPhPs), arising from the coupling of optical phonons and photons in the mid-IR regime, present a promising solution as long-range heat carriers capable of circumventing the limitations faced by traditional heat carriers such as acoustic phonons in nanoscales. However, the detection and utilization of SPhP-mediated thermal conduction have proven to be challenging. Here, we introduce an innovative approach that employs a grating-integrated thermometry platform, specifically designed to enhance the transmission of SPhP modes with long decay lengths and detectability of SPhPs over short, ballistic distances. We demonstrate quasi-ballistic, length-independent thermal conduction mediated by long-range SPhPs in one-dimensional SiO<sub>2</sub> heat channels, achieving a SPhP thermal conductivity of 1.5 W/m K, which has been over 90% of the intrinsic thermal conductivity.

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Publication Details

Journal
ACS Nano
Published
2025-05-29
DOI
https://doi.org/10.1021/acsnano.5c04594
Citations
4
Primary Topic
Thermal Radiation and Cooling Technologies
Type
article
Field-Weighted Citation Impact
3.81

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article

Quasi-Ballistic Heat Conduction of Long-Range Surface Phonon Polaritons Coupled to Thermal Reservoirs

Sunmi Shin, Rosmin Elsa Mohan, Hong‐Son Chu, Jingxuan Wang et al.
4 citations
ACS Nano
Thermal Radiation and Cooling Technologies
3.81
article

Quasi-Ballistic Heat Conduction of Long-Range Surface Phonon Polaritons Coupled to Thermal Reservoirs

Sunmi Shin, Rosmin Elsa Mohan, Hong‐Son Chu, Jingxuan Wang, Sichao Li
article en
4 citations

Abstract

Rigorous thermal control at the nanoscale has become essential with the miniaturization of electronic devices. However, heat transfer in such structures is hindered by increased boundary scatterings and reduced thermal conductivity. Surface phonon polaritons (SPhPs), arising from the coupling of optical phonons and photons in the mid-IR regime, present a promising solution as long-range heat carriers capable of circumventing the limitations faced by traditional heat carriers such as acoustic phonons in nanoscales. However, the detection and utilization of SPhP-mediated thermal conduction have proven to be challenging. Here, we introduce an innovative approach that employs a grating-integrated thermometry platform, specifically designed to enhance the transmission of SPhP modes with long decay lengths and detectability of SPhPs over short, ballistic distances. We demonstrate quasi-ballistic, length-independent thermal conduction mediated by long-range SPhPs in one-dimensional SiO<sub>2</sub> heat channels, achieving a SPhP thermal conductivity of 1.5 W/m K, which has been over 90% of the intrinsic thermal conductivity.

ACS NanoVol. 19(22)
Agency for Science, Technology and Research (SG), National University of Singapore (SG), Institute of High Performance Computing (SG), Faculty of Design (SI)
Ministry of Education - Singapore, Ministry of Trade, Industry and Energy
Affordable and clean energy
Openalex Percentile: Top 7%
Thermal Radiation and Cooling Technologies
3.81
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Quasi-Ballistic Heat Conduction of Long-Range Surface Phonon Polaritons Coupled to Thermal Reservoirs — Sunmi Shin, Rosmin Elsa Mohan, et al. · ACS Nano (2025) | TGRS Research Map | TGRS