Room-temperature exciton-polariton condensation in pressed perovskite microcavities

Abstract Microcavity exciton-polaritons, formed by strong light–matter coupling, are essential for realizing Bose–Einstein condensation and low-threshold lasing. Such polaritonic lasing and condensation have been demonstrated in III–V semiconductors at liquid helium temperatures. However, the complex fabrication of these microcavities and operating temperatures limit their room-temperature practical application. Here, we experimentally realize room-temperature exciton-polariton condensation and polaritonic lasing in a CsPbBr 3 perovskite planar microcavity fabricated by the pressing process. Angle-resolved photoluminescence spectra demonstrate the strong light–matter coupling and the formation of exciton-polaritons in such a pressed microcavity. Above the critical threshold, mass polaritons accumulating at the bottom of dispersion lead to a narrow emission linewidth and pronounced blueshift, further reinforcing the Bose–Einstein condensation and polaritonic lasing in this system. Our results offer a feasible and effective approach to investigate exciton-polariton condensation and polariton lasing at room temperature.

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Publication Details

Journal
Chinese Physics B
Published
2025-05-27
DOI
https://doi.org/10.1088/1674-1056/addce6
Primary Topic
Strong Light-Matter Interactions
Type
article
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article

Room-temperature exciton-polariton condensation in pressed perovskite microcavities

Wang Jun, Tianyin 天寅 Zhu 朱, Zelei 泽磊 Chen 陈, Zhongmin 钟民 Huang 黄 et al.
Chinese Physics B
Strong Light-Matter Interactions
article

Room-temperature exciton-polariton condensation in pressed perovskite microcavities

Wang Jun, Tianyin 天寅 Zhu 朱, Zelei 泽磊 Chen 陈, Zhongmin 钟民 Huang 黄, Xiaoyu 小宇 Wang 王, 赵海滨 Zhao Haibin
article en

Abstract

Abstract Microcavity exciton-polaritons, formed by strong light–matter coupling, are essential for realizing Bose–Einstein condensation and low-threshold lasing. Such polaritonic lasing and condensation have been demonstrated in III–V semiconductors at liquid helium temperatures. However, the complex fabrication of these microcavities and operating temperatures limit their room-temperature practical application. Here, we experimentally realize room-temperature exciton-polariton condensation and polaritonic lasing in a CsPbBr 3 perovskite planar microcavity fabricated by the pressing process. Angle-resolved photoluminescence spectra demonstrate the strong light–matter coupling and the formation of exciton-polaritons in such a pressed microcavity. Above the critical threshold, mass polaritons accumulating at the bottom of dispersion lead to a narrow emission linewidth and pronounced blueshift, further reinforcing the Bose–Einstein condensation and polaritonic lasing in this system. Our results offer a feasible and effective approach to investigate exciton-polariton condensation and polariton lasing at room temperature.

Chinese Physics BVol. 34(9)
Fudan University (CN)
Openalex Percentile: Top 91%
Strong Light-Matter Interactions
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