Effects of strain compensation on electron mobilities in InAs quantum wells grown on InP(001)

InAs quantum wells (QWs) grown on InP substrates are interesting for their applications in devices with high spin-orbit coupling and their potential role in creating topologically nontrivial hybrid heterostructures. These QWs rely on InGaAs cladding layers and InAlAs barrier layers to confine electrons within a thin InAs well. The highest mobility QWs are limited by interfacial roughness scattering and alloy disorder scattering in the cladding and barrier layers. Increasing QW thickness has been shown to reduce the effect of both of these scattering mechanisms. However, for current state-of-the-art devices with As-based cladding and barrier layers, the critical thickness is limited to $\ensuremath{\le}7$ nm. In this paper, we demonstrate the use of strain compensation techniques in the ${\mathrm{In}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}$ cladding layers, grown on ${\mathrm{In}}_{0.81}{\mathrm{Al}}_{0.19}\mathrm{As}$ barrier layers, to extend the critical thickness well beyond this limit. We induce tensile strain in the InGaAs cladding layers by reducing the In concentration from ${\mathrm{In}}_{0.81}{\mathrm{Ga}}_{0.19}\mathrm{As}$ to ${\mathrm{In}}_{0.70}{\mathrm{Ga}}_{0.30}\mathrm{As}$ and we observe changes in both the critical thickness of the well and the maximum achievable mobility. The peak electron mobility at 2 K is $1.16\ifmmode\times\else\texttimes\fi{}{10}^{6}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{2}/\mathrm{V}\phantom{\rule{0.16em}{0ex}}\mathrm{s}$, with a carrier density of $4.2\ifmmode\times\else\texttimes\fi{}{10}^{11}\phantom{\rule{0.16em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}2}$. Additionally, we study the quantum lifetime and Rashba spin splitting in the highest mobility device as these parameters are critical to determine if these structures can be used in topologically nontrivial devices.

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Publication Details

Journal
Physical Review Materials
Published
2025-05-27
DOI
https://doi.org/10.1103/physrevmaterials.9.054607
Citations
1
Primary Topic
Semiconductor Quantum Structures and Devices
Type
article
Field-Weighted Citation Impact
1.25

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article

Effects of strain compensation on electron mobilities in InAs quantum wells grown on InP(001)

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Physical Review Materials
Semiconductor Quantum Structures and Devices
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article

Effects of strain compensation on electron mobilities in InAs quantum wells grown on InP(001)

Y. Gul, Connor P. Dempsey, C. J. Palmstrøm, S. N. Holmes, Jason T. Dong, Mihir Pendharkar, M. Pepper, I. Villar Rodriguez, S Chatterjee
article en
1 citations

Abstract

InAs quantum wells (QWs) grown on InP substrates are interesting for their applications in devices with high spin-orbit coupling and their potential role in creating topologically nontrivial hybrid heterostructures. These QWs rely on InGaAs cladding layers and InAlAs barrier layers to confine electrons within a thin InAs well. The highest mobility QWs are limited by interfacial roughness scattering and alloy disorder scattering in the cladding and barrier layers. Increasing QW thickness has been shown to reduce the effect of both of these scattering mechanisms. However, for current state-of-the-art devices with As-based cladding and barrier layers, the critical thickness is limited to $\ensuremath{\le}7$ nm. In this paper, we demonstrate the use of strain compensation techniques in the ${\mathrm{In}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}$ cladding layers, grown on ${\mathrm{In}}_{0.81}{\mathrm{Al}}_{0.19}\mathrm{As}$ barrier layers, to extend the critical thickness well beyond this limit. We induce tensile strain in the InGaAs cladding layers by reducing the In concentration from ${\mathrm{In}}_{0.81}{\mathrm{Ga}}_{0.19}\mathrm{As}$ to ${\mathrm{In}}_{0.70}{\mathrm{Ga}}_{0.30}\mathrm{As}$ and we observe changes in both the critical thickness of the well and the maximum achievable mobility. The peak electron mobility at 2 K is $1.16\ifmmode\times\else\texttimes\fi{}{10}^{6}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{2}/\mathrm{V}\phantom{\rule{0.16em}{0ex}}\mathrm{s}$, with a carrier density of $4.2\ifmmode\times\else\texttimes\fi{}{10}^{11}\phantom{\rule{0.16em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}2}$. Additionally, we study the quantum lifetime and Rashba spin splitting in the highest mobility device as these parameters are critical to determine if these structures can be used in topologically nontrivial devices.

Physical Review MaterialsVol. 9(5)
University of California, Santa Barbara (US), London Centre for Nanotechnology (GB), University College London (GB)
National Science Foundation, U.S. Department of Energy, Science and Technology Facilities Council
Openalex Percentile: Top 21%
Semiconductor Quantum Structures and Devices
1.25
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