Contrasting Mechanisms Controlling Pb Isotopes of Dust in Inland and Marine Archives

Abstract Lead (Pb) isotopes are powerful tools for tracing dust provenance and reconstructing paleoclimate. However, variations in Pb isotopic compositions among different grain‐size fractions in sediments complicate their use. We examine the Nd‐Pb isotopic compositions of two sediment fractions (<2 μm and 30–63 μm) from the central Japan Sea during the last glaciation (26–12 ka BP). Our results indicate that these sediments primarily consist of aeolian dust transported by the East Asian Winter Monsoon. The <2 μm fraction exhibits more radiogenic Pb isotopes than the 30–63 μm fraction. This size‐dependent discrepancy in Pb isotopes is attributed to differences in sediment composition, governed by the incongruent weathering of minerals in source rocks and transport sorting. Comparisons of dust records from inland and marine archives reveal contrasting mechanisms that control Pb isotopic compositions. We propose that greater caution is necessary when using Pb isotopes in paleoclimatology and paleoceanography.

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Publication Details

Journal
Geophysical Research Letters
Published
2025-05-24
DOI
https://doi.org/10.1029/2024gl114133
Primary Topic
Geology and Paleoclimatology Research
Type
article
Field-Weighted Citation Impact
0.00

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article

Contrasting Mechanisms Controlling Pb Isotopes of Dust in Inland and Marine Archives

Xuefa Shi, Aleksandr A. Bosin, Yuriy P. Vasilenko, Ruxi Dou et al.
Geophysical Research Letters
Geology and Paleoclimatology Research
article

Contrasting Mechanisms Controlling Pb Isotopes of Dust in Inland and Marine Archives

Xuefa Shi, Aleksandr A. Bosin, Yuriy P. Vasilenko, Ruxi Dou, Xinqing Zou, Sergey A. Gorbarenko, Jianjun Zou, Yonghua Wu, Aimei Zhu, Xuguang Feng, Zhi Dong
article en

Abstract

Abstract Lead (Pb) isotopes are powerful tools for tracing dust provenance and reconstructing paleoclimate. However, variations in Pb isotopic compositions among different grain‐size fractions in sediments complicate their use. We examine the Nd‐Pb isotopic compositions of two sediment fractions (<2 μm and 30–63 μm) from the central Japan Sea during the last glaciation (26–12 ka BP). Our results indicate that these sediments primarily consist of aeolian dust transported by the East Asian Winter Monsoon. The <2 μm fraction exhibits more radiogenic Pb isotopes than the 30–63 μm fraction. This size‐dependent discrepancy in Pb isotopes is attributed to differences in sediment composition, governed by the incongruent weathering of minerals in source rocks and transport sorting. Comparisons of dust records from inland and marine archives reveal contrasting mechanisms that control Pb isotopic compositions. We propose that greater caution is necessary when using Pb isotopes in paleoclimatology and paleoceanography.

Geophysical Research LettersVol. 52(10)
Russian Academy of Sciences (RU), Ministry of Natural Resources (CN), Qingdao National Laboratory for Marine Science and Technology (CN), First Institute of Oceanography (CN), Jiangsu Center for Collaborative Innovation in Geographical Information Resource Development and Application (CN), V.I. Il'ichev Pacific Oceanological Institute (RU), Nanjing University (CN)
National Natural Science Foundation of China, Ministry of Education and Science of the Russian Federation, National Natural Science Foundation of China-Shandong Joint Fund, National Key Research and Development Program of China
Openalex Percentile: Top 84%
Geology and Paleoclimatology Research
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