Glass transition in metallic glasses facilitated by static loading

The glass transition represents a long-standing enigma in condensed matter physics and materials science. Traditionally, this transition, often associated with \ensuremath{\alpha} relaxation, is viewed as a thermally activated process. In this study, by integrating molecular dynamics simulations and experimental verification, we revealed that static loading can effectively reduce the glass transition temperature in the out-of-equilibrium glassy state, exhibiting a distinct stress-temperature equivalence compared to that observed under dynamic loading in the equilibrium liquid state. This indicates that mechanical energy can effectively substitute thermal energy in facilitating the glass transition. At the microscopic level, the application of static load enhances atomic mobility, triggering cooperative atomic movements and fostering the development of ``faster-atom'' networks, which ultimately facilitate the global motion of numerous atoms necessary for the glass transition. These findings highlight the significance of static load in tailoring the structure and dynamics of metallic glasses.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-05-22
DOI
https://doi.org/10.1103/physrevb.111.184107
Citations
3
Primary Topic
Metallic Glasses and Amorphous Alloys
Type
article
Field-Weighted Citation Impact
2.14

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article

Glass transition in metallic glasses facilitated by static loading

Hongbo Zhou, Huaping Zhang, Chao Cheng Chang, Weihua Wang et al.
3 citations
Physical review. B./Physical review. B
Metallic Glasses and Amorphous Alloys
2.14
article

Glass transition in metallic glasses facilitated by static loading

Hongbo Zhou, Huaping Zhang, Chao Cheng Chang, Weihua Wang, Huawei Sun, Minqiang Jiang
article en
3 citations

Abstract

The glass transition represents a long-standing enigma in condensed matter physics and materials science. Traditionally, this transition, often associated with \ensuremath{\alpha} relaxation, is viewed as a thermally activated process. In this study, by integrating molecular dynamics simulations and experimental verification, we revealed that static loading can effectively reduce the glass transition temperature in the out-of-equilibrium glassy state, exhibiting a distinct stress-temperature equivalence compared to that observed under dynamic loading in the equilibrium liquid state. This indicates that mechanical energy can effectively substitute thermal energy in facilitating the glass transition. At the microscopic level, the application of static load enhances atomic mobility, triggering cooperative atomic movements and fostering the development of ``faster-atom'' networks, which ultimately facilitate the global motion of numerous atoms necessary for the glass transition. These findings highlight the significance of static load in tailoring the structure and dynamics of metallic glasses.

Physical review. B./Physical review. BVol. 111(18)
Chinese Academy of Sciences (CN), Songshan Lake Materials Laboratory (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), University of Chinese Academy of Sciences (CN)
National Natural Science Foundation of China, Chinese Academy of Sciences, Basic and Applied Basic Research Foundation of Guangdong Province
Openalex Percentile: Top 14%
Metallic Glasses and Amorphous Alloys
2.14
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