Phase-Resolved Attoclock

How long an electron spends under the barrier during strong field tunneling ionization is still a controversial issue in attosecond science. We develop a new attoclock technique to address this problem. It exploits the carrier-envelope-phase dependence of angular streaking to extrapolate from elliptically polarized light measurements, for the first time, the deflection angles for circularly polarized light. Thus, we can avoid the ambiguity inherent to the modeling of the conventional elliptical attoclock. Our results show that the deflection angles are solely sensitive to the ionization potentials of targets and tunneling delay is a minor effect.

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Publication Details

Journal
Physical Review Letters
Published
2025-05-20
DOI
https://doi.org/10.1103/physrevlett.134.203201
Citations
2
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
2.49

Funders

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article

Phase-Resolved Attoclock

Emmanuel Orunesajo, Richard Taïeb, Jonathan Dubois, Sulaiman Abubakar et al.
2 citations
Physical Review Letters
Laser-Matter Interactions and Applications
2.49
article

Phase-Resolved Attoclock

Emmanuel Orunesajo, Richard Taïeb, Jonathan Dubois, Sulaiman Abubakar, Suk Kyoung Lee, Léonardo Rico, Yasashri Ranathunga, Wen Li, Blessed Oguh
article en
2 citations

Abstract

How long an electron spends under the barrier during strong field tunneling ionization is still a controversial issue in attosecond science. We develop a new attoclock technique to address this problem. It exploits the carrier-envelope-phase dependence of angular streaking to extrapolate from elliptically polarized light measurements, for the first time, the deflection angles for circularly polarized light. Thus, we can avoid the ambiguity inherent to the modeling of the conventional elliptical attoclock. Our results show that the deflection angles are solely sensitive to the ionization potentials of targets and tunneling delay is a minor effect.

Physical Review LettersVol. 134(20)
Wayne State University (US), Sorbonne Université (FR), Laboratoire de Chimie Physique - Matière et Rayonnement (FR), Laboratoire Médiations (FR)
National Science Foundation, U.S. Department of Energy, Agence Nationale de la Recherche, H2020 Marie Skłodowska-Curie Actions
Openalex Percentile: Top 12%
Laser-Matter Interactions and Applications
2.49
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