Phase-space Gaussian quantum ensemble for high-order harmonic generation

We propose a phase-space Gaussian quantum ensemble to depict the high-order harmonic generation process. Our model takes the wave-particle duality and the uncertainty principle into account. It bridges the ab initio calculation with the semiclassical analysis, enabling us to distinguish different channels and reveal the underlying electron dynamics. We investigate the ionization and recombination time of the short, long, and multi-rescattering trajectory harmonics. Our model also provides access to investigate the position-momentum properties. Results demonstrate that the electron has a nonzero initial velocity at the tunnel exit, revealing the nonadiabatic effect. We prove the validity of our analysis by interpreting the observables in the two-color interference experiments. The nonzero transverse harmonic signal for any two-color delay in the orthogonally polarized fields can be explained by the delocalized distribution of the quantum ensemble. Our model can guide the semiclassical analysis and provide a benchmark for high-order harmonic spectroscopy.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-05-20
DOI
https://doi.org/10.1103/physreva.111.053114
Citations
1
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
1.25

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article

Phase-space Gaussian quantum ensemble for high-order harmonic generation

Pengfei Lan, Sen Qiao, Hubin Cui, Liang Li et al.
1 citations
Physical review. A/Physical review, A
Laser-Matter Interactions and Applications
1.25
article

Phase-space Gaussian quantum ensemble for high-order harmonic generation

Pengfei Lan, Sen Qiao, Hubin Cui, Liang Li, Peixiang Lu, Shiqi Liang, S. Zeng
article en
1 citations

Abstract

We propose a phase-space Gaussian quantum ensemble to depict the high-order harmonic generation process. Our model takes the wave-particle duality and the uncertainty principle into account. It bridges the ab initio calculation with the semiclassical analysis, enabling us to distinguish different channels and reveal the underlying electron dynamics. We investigate the ionization and recombination time of the short, long, and multi-rescattering trajectory harmonics. Our model also provides access to investigate the position-momentum properties. Results demonstrate that the electron has a nonzero initial velocity at the tunnel exit, revealing the nonadiabatic effect. We prove the validity of our analysis by interpreting the observables in the two-color interference experiments. The nonzero transverse harmonic signal for any two-color delay in the orthogonally polarized fields can be explained by the delocalized distribution of the quantum ensemble. Our model can guide the semiclassical analysis and provide a benchmark for high-order harmonic spectroscopy.

Physical review. A/Physical review, AVol. 111(5)
Yangtze Optical Electronic (China) (CN), Huazhong University of Science and Technology (CN)
National Natural Science Foundation of China, Huazhong University of Science and Technology, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 21%
Laser-Matter Interactions and Applications
1.25
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Phase-space Gaussian quantum ensemble for high-order harmonic generation — Pengfei Lan, Sen Qiao, et al. · Physical review. A/Physical review, A (2025) | TGRS Research Map | TGRS