A rate dependent interface model for stick-slip fracture in adhesives and polymer glasses

In stick-slip fracture, a crack stays still or only propagates a small amount until it reaches a critical energy release rate. Then, it suddenly grows rapidly, causing the energy release rate to drop and the crack to stop again. This behavior is common in many polymers, including glassy polymers and soft materials like adhesives. However, the theoretical understanding of this phenomenon is fragmented and incomplete. Here we propose a unified theory based on a rate-dependent cohesive model to explain these phenomena. Using this model, we demonstrate that an elastic backing layer in a zero-degree peel test can experience different types of stick-slip instability depending on the peeling rate. At slow peeling rates, the crack grows slowly until it reaches a maximum velocity, corresponding to a fixed maximum force, after which the growth becomes unstable. However, above a certain critical peeling rate, there is no slow crack growth: the crack enters the stick-slip regime once the critical energy release rate is reached for a reduced value of the applied force. Although our mathematical modeling is developed in a specific geometry that makes the computations easier, this behavior can be argued to be a more general feature of most materials and geometries presenting stick-slip fracture.

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Publication Details

Journal
Soft Matter
Published
2025-01-01
DOI
https://doi.org/10.1039/d4sm01433b
Citations
2
Primary Topic
Mechanical Behavior of Composites
Type
article
Field-Weighted Citation Impact
1.73

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article

A rate dependent interface model for stick-slip fracture in adhesives and polymer glasses

Chung‐Yuen Hui, Matteo Ciccotti, Xuemei Xiao
2 citations
Soft Matter
Mechanical Behavior of Composites
1.73
article

A rate dependent interface model for stick-slip fracture in adhesives and polymer glasses

Chung‐Yuen Hui, Matteo Ciccotti, Xuemei Xiao
article en
2 citations

Abstract

In stick-slip fracture, a crack stays still or only propagates a small amount until it reaches a critical energy release rate. Then, it suddenly grows rapidly, causing the energy release rate to drop and the crack to stop again. This behavior is common in many polymers, including glassy polymers and soft materials like adhesives. However, the theoretical understanding of this phenomenon is fragmented and incomplete. Here we propose a unified theory based on a rate-dependent cohesive model to explain these phenomena. Using this model, we demonstrate that an elastic backing layer in a zero-degree peel test can experience different types of stick-slip instability depending on the peeling rate. At slow peeling rates, the crack grows slowly until it reaches a maximum velocity, corresponding to a fixed maximum force, after which the growth becomes unstable. However, above a certain critical peeling rate, there is no slow crack growth: the crack enters the stick-slip regime once the critical energy release rate is reached for a reduced value of the applied force. Although our mathematical modeling is developed in a specific geometry that makes the computations easier, this behavior can be argued to be a more general feature of most materials and geometries presenting stick-slip fracture.

Soft MatterVol. 21(26)
Centre National de la Recherche Scientifique (FR), Hokkaido University (JP), Cornell University (US), Université Paris Sciences et Lettres (FR), Sorbonne Université (FR), Sciences et Ingénierie de la Matière Molle (FR), ESPCI Paris (FR)
National Science Foundation, Agence Nationale de la Recherche
Affordable and clean energy
Openalex Percentile: Top 18%
Mechanical Behavior of Composites
1.73
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A rate dependent interface model for stick-slip fracture in adhesives and polymer glasses — Chung‐Yuen Hui, Matteo Ciccotti, et al. · Soft Matter (2025) | TGRS Research Map | TGRS