Inkjet-Printed Flexible Piezoelectric Sensor for Large Deformation Applications

Next-generation flexible, soft, and stretchable sensors and electronic devices are conquering the technological scene due to their extremely innovative applications. Especially when produced via innovative technologies like additive manufacturing (AM) and/or inkjet printing (IJP), they represent an undeniable strategic asset for Industry 5.0. Within the growing sensor market, they offer advantages in terms of sensitivity and maximum sensing range. In addition, the use of AM/IJP reduces material waste, enhances scalability, and lowers cost production. In the present work, the design and fabrication of a highly flexible inkjet-printed piezoelectric sensor on top of a thin highly flexible polyimide substrate are presented. The silver top and bottom electrodes were inkjet-printed together with a P(VDF-TrFE) active layer with a nominal thickness of 3 μm which is located between them. The experimental results demonstrate that, even in extreme bending conditions and at different bending speeds, the fabricated sensors are able to maintain their performance without mechanical delamination, giving a stable and repeatable output peak-to-peak signal of 850 mV under cyclic bending. The material combination and the IJP-based fabrication technique employed for the first time in this work to produce highly flexible sensors represent a promising novelty in terms of both sensor performance and customization possibilities.