Concurrence of in-plane anisotropic superconductivity and quasi-one-dimensional charge density wave in layered CuTe under high pressure

Despite its layered orthorhombic lattice structure, CuTe hosts quasi-one-dimensional (quasi-1D) charge density wave (CDW) distortions of in-plane Te chains along the $a$ axis below ${T}_{\mathrm{CDW}}\ensuremath{\sim}346\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. This unique quasi-1D CDW manifests itself as an in-plane resistivity anisotropy, i.e., the $a$-axis resistivity (${\ensuremath{\rho}}_{a}$) displays an evident humplike anomaly below ${T}_{\mathrm{CDW}}$ while the $b$-axis resistivity (${\ensuremath{\rho}}_{b}$) is featureless. Herein, we present simultaneous measurements of ${\ensuremath{\rho}}_{a}$ and ${\ensuremath{\rho}}_{b}$ at various pressures to 16.0 GPa, in order to trace the quasi-1D CDW's evolution and its interplay with the induced superconductivity (SC). We found no sign of SC at ambient pressure from ${\ensuremath{\rho}}_{a}$ and ${\ensuremath{\rho}}_{b}$ with temperatures down to as low as 0.05 K. With the application of pressure, ${T}_{\mathrm{CDW}}$ from ${\ensuremath{\rho}}_{a}$ deceases linearly yet the quasi-1D CDW character of CuTe keeps unchanged with pressures to 6.4 GPa, above which it breaks down due to the formation of an isotropic electronic interaction-driven CDW. Meanwhile, a local superconducting pairing starts to nucleate at 3.9 GPa initially within the preexisting quasi-1D CDW Te chains (along the $a$ axis) at \ensuremath{\sim}0.4 K. For a given higher pressure, distinct discrepancies in the zero-resistance temperature and the upper critical field are observed, both of which disappear suddenly along with the CDW transformation. Such a rare observation of the in-plane anisotropic SC interlocking with the quasi-1D CDW in pressurized CuTe has been discussed in terms of the particular fermiology, local superconducting pairing, and strong CDW fluctuations that are all rooted in the quasi-1D, chainlike arrangement of its in-plane Te atoms.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-05-19
DOI
https://doi.org/10.1103/physrevb.111.l180507
Primary Topic
Organic and Molecular Conductors Research
Type
article
Field-Weighted Citation Impact
0.00

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article

Concurrence of in-plane anisotropic superconductivity and quasi-one-dimensional charge density wave in layered CuTe under high pressure

Yonghui Zhou, Ning Hao, Xuliang Chen, Shuyang Wang et al.
Physical review. B./Physical review. B
Organic and Molecular Conductors Research
article

Concurrence of in-plane anisotropic superconductivity and quasi-one-dimensional charge density wave in layered CuTe under high pressure

Yonghui Zhou, Ning Hao, Xuliang Chen, Shuyang Wang, Chao An, Yusheng Shi, Zhaorong Yang, Qing Wang
article en

Abstract

Despite its layered orthorhombic lattice structure, CuTe hosts quasi-one-dimensional (quasi-1D) charge density wave (CDW) distortions of in-plane Te chains along the $a$ axis below ${T}_{\mathrm{CDW}}\ensuremath{\sim}346\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. This unique quasi-1D CDW manifests itself as an in-plane resistivity anisotropy, i.e., the $a$-axis resistivity (${\ensuremath{\rho}}_{a}$) displays an evident humplike anomaly below ${T}_{\mathrm{CDW}}$ while the $b$-axis resistivity (${\ensuremath{\rho}}_{b}$) is featureless. Herein, we present simultaneous measurements of ${\ensuremath{\rho}}_{a}$ and ${\ensuremath{\rho}}_{b}$ at various pressures to 16.0 GPa, in order to trace the quasi-1D CDW's evolution and its interplay with the induced superconductivity (SC). We found no sign of SC at ambient pressure from ${\ensuremath{\rho}}_{a}$ and ${\ensuremath{\rho}}_{b}$ with temperatures down to as low as 0.05 K. With the application of pressure, ${T}_{\mathrm{CDW}}$ from ${\ensuremath{\rho}}_{a}$ deceases linearly yet the quasi-1D CDW character of CuTe keeps unchanged with pressures to 6.4 GPa, above which it breaks down due to the formation of an isotropic electronic interaction-driven CDW. Meanwhile, a local superconducting pairing starts to nucleate at 3.9 GPa initially within the preexisting quasi-1D CDW Te chains (along the $a$ axis) at \ensuremath{\sim}0.4 K. For a given higher pressure, distinct discrepancies in the zero-resistance temperature and the upper critical field are observed, both of which disappear suddenly along with the CDW transformation. Such a rare observation of the in-plane anisotropic SC interlocking with the quasi-1D CDW in pressurized CuTe has been discussed in terms of the particular fermiology, local superconducting pairing, and strong CDW fluctuations that are all rooted in the quasi-1D, chainlike arrangement of its in-plane Te atoms.

Physical review. B./Physical review. BVol. 111(18)
Anhui University (CN), High Magnetic Field Laboratory (CN)
National Natural Science Foundation of China, Chinese Academy of Sciences, China Postdoctoral Science Foundation, Natural Science Foundation of Anhui Province, National Key Research and Development Program of China
Climate action
Openalex Percentile: Top 94%
Organic and Molecular Conductors Research
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