Cavity Spectroscopy for Strongly Correlated Polaritonic Systems
Embedding materials in optical cavities has emerged as an intriguing perspective for controlling quantum materials, but a key challenge lies in measuring properties of the embedded matter. Here, we propose a framework for probing strongly correlated cavity-embedded materials through direct measurements of cavity photons. We derive general relations between photon and matter observables inside the cavity, and show how these can be measured via the emitted photons. As an example, we demonstrate how the entanglement phase transition of an embedded H_{2} molecule can be accessed by measuring the cavity photon occupation, and showcase how dynamical spin correlation functions can be accessed by measuring dynamical photon correlation functions. Our framework provides an all-optical method to measure static and dynamic properties of cavity-embedded materials.
Authors
- Dante Marvin Kennes (ORCID: https://orcid.org/0000-0002-9838-6866)
- Mark Kamper Svendsen (ORCID: https://orcid.org/0000-0001-9718-849X)
- Emil Viñas Boström (ORCID: https://orcid.org/0000-0002-3318-4454)
- Ángel Rubio (ORCID: https://orcid.org/0000-0003-2060-3151)
- Karl J. Friston
Institutions
- University of the Basque Country (ES)
- Max Planck Institute for the Structure and Dynamics of Matter (DE)
- Flatiron Health (United States) (US)
- Flatiron Institute (US)
- RWTH Aachen University (DE)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2025-05-16
- DOI
- https://doi.org/10.1103/1lpw-22np
- Citations
- 2
- Primary Topic
- Strong Light-Matter Interactions
- Type
- article
- Field-Weighted Citation Impact
- 2.49
Funders
- Flatiron Health
- European Commission
- Deutsche Forschungsgemeinschaft
- Novo Nordisk
- Novo Nordisk Fonden
- Horizon 2020 Framework Programme
- HORIZON EUROPE Framework Programme
- HORIZON EUROPE Marie Sklodowska-Curie Actions