Cavity Spectroscopy for Strongly Correlated Polaritonic Systems

Embedding materials in optical cavities has emerged as an intriguing perspective for controlling quantum materials, but a key challenge lies in measuring properties of the embedded matter. Here, we propose a framework for probing strongly correlated cavity-embedded materials through direct measurements of cavity photons. We derive general relations between photon and matter observables inside the cavity, and show how these can be measured via the emitted photons. As an example, we demonstrate how the entanglement phase transition of an embedded H_{2} molecule can be accessed by measuring the cavity photon occupation, and showcase how dynamical spin correlation functions can be accessed by measuring dynamical photon correlation functions. Our framework provides an all-optical method to measure static and dynamic properties of cavity-embedded materials.

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Publication Details

Journal
Physical Review Letters
Published
2025-05-16
DOI
https://doi.org/10.1103/1lpw-22np
Citations
2
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
2.49

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Cavity Spectroscopy for Strongly Correlated Polaritonic Systems

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article

Cavity Spectroscopy for Strongly Correlated Polaritonic Systems

Dante Marvin Kennes, Mark Kamper Svendsen, Emil Viñas Boström, Ángel Rubio, Karl J. Friston
article en
2 citations

Abstract

Embedding materials in optical cavities has emerged as an intriguing perspective for controlling quantum materials, but a key challenge lies in measuring properties of the embedded matter. Here, we propose a framework for probing strongly correlated cavity-embedded materials through direct measurements of cavity photons. We derive general relations between photon and matter observables inside the cavity, and show how these can be measured via the emitted photons. As an example, we demonstrate how the entanglement phase transition of an embedded H_{2} molecule can be accessed by measuring the cavity photon occupation, and showcase how dynamical spin correlation functions can be accessed by measuring dynamical photon correlation functions. Our framework provides an all-optical method to measure static and dynamic properties of cavity-embedded materials.

Physical Review LettersVol. 134(24)
University of the Basque Country (ES), Max Planck Institute for the Structure and Dynamics of Matter (DE), Flatiron Health (United States) (US), Flatiron Institute (US), RWTH Aachen University (DE)
Flatiron Health, European Commission, Deutsche Forschungsgemeinschaft, Novo Nordisk, Novo Nordisk Fonden, Horizon 2020 Framework Programme, HORIZON EUROPE Framework Programme, HORIZON EUROPE Marie Sklodowska-Curie Actions
Climate action
Openalex Percentile: Top 12%
Strong Light-Matter Interactions
2.49
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