Cost-Efficient Deterministic Engineering of Single Photon Emitters in Two-Dimensional Materials

Two-dimensional materials have recently emerged as promising candidates for quantum light emission. Their tunable bandgaps, layer-dependent excitonic properties, and strong confinement of charge carriers provide a versatile platform for manipulating and controlling quantum states. Several approaches─such as strain engineering, defect engineering and surface functionalization─have been explored to induce single-photon emitters in these materials. In this work, we present a practical and cost-efficient methodology for deterministic strain engineering of single-photon emitters within thin flakes of GaSe. Our approach utilizes optically active microparticles with a distinctive bipyramidal shape, whose emission does not interfere optically with that of GaSe. The results show strong agreement with previous studies on strain-induced single-photon sources in multilayer GaSe, demonstrating that the proposed technique is a promising platform for generating nonclassical light emission in layered materials. Compared to other local strain engineering techniques for single-photon sources in two-dimensional materials, our method offers greater accessibility and lower cost, making it feasible for implementation in most laboratories performing the experimental research in the field. This increased accessibility can help advance the understanding of two-dimensional semiconductor systems and their potential applications in nanophotonics and quantum light technologies.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2025-05-15
DOI
https://doi.org/10.1021/acsami.5c05174
Primary Topic
Nanowire Synthesis and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Cost-Efficient Deterministic Engineering of Single Photon Emitters in Two-Dimensional Materials

Sanja Djurdjić Mijin, S. Lazić, Eva Hemmer, Nikita Panov et al.
ACS Applied Materials & Interfaces
Nanowire Synthesis and Applications
article

Cost-Efficient Deterministic Engineering of Single Photon Emitters in Two-Dimensional Materials

Sanja Djurdjić Mijin, S. Lazić, Eva Hemmer, Nikita Panov, Ismael dePedro-Embid
article en

Abstract

Two-dimensional materials have recently emerged as promising candidates for quantum light emission. Their tunable bandgaps, layer-dependent excitonic properties, and strong confinement of charge carriers provide a versatile platform for manipulating and controlling quantum states. Several approaches─such as strain engineering, defect engineering and surface functionalization─have been explored to induce single-photon emitters in these materials. In this work, we present a practical and cost-efficient methodology for deterministic strain engineering of single-photon emitters within thin flakes of GaSe. Our approach utilizes optically active microparticles with a distinctive bipyramidal shape, whose emission does not interfere optically with that of GaSe. The results show strong agreement with previous studies on strain-induced single-photon sources in multilayer GaSe, demonstrating that the proposed technique is a promising platform for generating nonclassical light emission in layered materials. Compared to other local strain engineering techniques for single-photon sources in two-dimensional materials, our method offers greater accessibility and lower cost, making it feasible for implementation in most laboratories performing the experimental research in the field. This increased accessibility can help advance the understanding of two-dimensional semiconductor systems and their potential applications in nanophotonics and quantum light technologies.

ACS Applied Materials & InterfacesVol. 17(21)
University of Ottawa (CA), University of Belgrade (RS), Paul Drude Institute for Solid State Electronics (DE), Institute of Physics Belgrade (RS), Forschungsverbund Berlin (DE), Universidad Autónoma de Madrid (ES)
Ministerio de Ciencia, Innovación y Universidades
Openalex Percentile: Top 90%
Nanowire Synthesis and Applications
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