A Unified Equation for Predicting Crack Growth in Rubber Composites Across All Crack Growth Rates

The relationship between tearing energy and crack growth rates in elastomers is typically divided into three regions-slow crack growth, fast crack growth, and a transitional region-each described by separate power law relationships, requiring six variables to fully characterize the behavior. This study introduces a novel, unified equation that simplifies this relationship by combining two coexisting energy dissipation mechanisms into a single model with only four variables. The model consists of two terms, one for each energy dissipation mechanism: one term is dominant at slow crack growth rates and limited by a threshold energy, and the other is dominant at fast speeds. The transition region emerges naturally as the dominant mechanism shifts. The model's simplicity enables new advances, such as predicting fast crack growth tearing and transition energies using only slow crack growth data. This capability is demonstrated across a wide range of non-strain crystallizing rubbers, including filled and unfilled compounds, tested at room temperature and elevated temperatures and in both swollen and unswollen states. This model offers a practical tool for material design, failure prediction, and reducing experimental effort in characterizing elastomer performance. Notably, this is the first model to unify slow, transition, and fast crack growth regimes into a single continuous equation requiring only four variables, enabling the prediction of high-speed behavior using only low-speed experimental data-a major advantage over existing six-parameter models.

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Publication Details

Journal
Polymers
Published
2025-05-15
DOI
https://doi.org/10.3390/polym17101357
Primary Topic
Elasticity and Material Modeling
Type
article
Field-Weighted Citation Impact
0.00

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article

A Unified Equation for Predicting Crack Growth in Rubber Composites Across All Crack Growth Rates

Keizo Akutagawa, James J. C. Busfield, Dimitrios G. Papageorgiou, Aaron M. Duncan et al.
Polymers
Elasticity and Material Modeling
article

A Unified Equation for Predicting Crack Growth in Rubber Composites Across All Crack Growth Rates

Keizo Akutagawa, James J. C. Busfield, Dimitrios G. Papageorgiou, Aaron M. Duncan, Julien Ramier
article en

Abstract

The relationship between tearing energy and crack growth rates in elastomers is typically divided into three regions-slow crack growth, fast crack growth, and a transitional region-each described by separate power law relationships, requiring six variables to fully characterize the behavior. This study introduces a novel, unified equation that simplifies this relationship by combining two coexisting energy dissipation mechanisms into a single model with only four variables. The model consists of two terms, one for each energy dissipation mechanism: one term is dominant at slow crack growth rates and limited by a threshold energy, and the other is dominant at fast speeds. The transition region emerges naturally as the dominant mechanism shifts. The model's simplicity enables new advances, such as predicting fast crack growth tearing and transition energies using only slow crack growth data. This capability is demonstrated across a wide range of non-strain crystallizing rubbers, including filled and unfilled compounds, tested at room temperature and elevated temperatures and in both swollen and unswollen states. This model offers a practical tool for material design, failure prediction, and reducing experimental effort in characterizing elastomer performance. Notably, this is the first model to unify slow, transition, and fast crack growth regimes into a single continuous equation requiring only four variables, enabling the prediction of high-speed behavior using only low-speed experimental data-a major advantage over existing six-parameter models.

PolymersVol. 17(10)
Queen Mary University of London (GB)
Engineering and Physical Sciences Research Council
Openalex Percentile: Top 90%
Elasticity and Material Modeling
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A Unified Equation for Predicting Crack Growth in Rubber Composites Across All Crack Growth Rates — Keizo Akutagawa, James J. C. Busfield, et al. · Polymers (2025) | TGRS Research Map | TGRS