Enhanced coherence from correlated states in WSe2/MoS2 moiré heterobilayer
Moiré superlattices in van der Waals materials have emerged as a promising platform for studying the correlated states in condensed matter physics. These correlated states have substantial effects on the emission coherence, an important parameter for quantum light applications. However, the effect of correlated states on the excitonic emission coherence is largely unexplored. Here, we show that the coherence of moiré interlayer exciton emission in tungsten diselenide (WSe<sub>2</sub>)/molybdenum disulfide (MoS<sub>2</sub>) heterobilayers is sensitive to the correlated insulating states in this material. We demonstrate that the emission linewidth of interlayer exciton shows a dip at a particular power range, which we attributed to the excitonic (bosonic) interaction. Moreover, such linewidth minima also appear in the doping dependence of the photoluminescence spectrum at the integer electronic filling factor, f<sub>el</sub> = 1, demonstrating the effect of the electronic (fermionic) correlated insulating state on the interlayer exciton emission coherence. Our results demonstrate the richness of exciton-exciton and exciton-electron interactions in moiré semiconductors and pave the way for engineering emission coherence by controlling such interactions.
Authors
- Qinghai Tan (ORCID: https://orcid.org/0000-0003-4808-4795)
- Takashi Taniguchi (ORCID: https://orcid.org/0000-0002-1467-3105)
- Kenji Watanabe (ORCID: https://orcid.org/0000-0003-3701-8119)
- Ruihua He (ORCID: https://orcid.org/0000-0003-3235-1991)
- Abdullah Rasmita (ORCID: https://orcid.org/0000-0002-0669-7131)
- Hongbing Cai (ORCID: https://orcid.org/0000-0003-3186-1041)
- Weibo Gao (ORCID: https://orcid.org/0000-0003-3971-621X)
- Xiangbin Cai
- Zhaowei Zhang (ORCID: https://orcid.org/0000-0002-0603-6763)
- Xuran Dai (ORCID: https://orcid.org/0000-0003-1818-2335)
Institutions
- Centre for Quantum Technologies (SG)
- University of Science and Technology of China (CN)
- Nanyang Technological University (SG)
- National Institute for Materials Science (JP)
- Quantum Design (Germany) (DE)
Publication Details
- Journal
- Nature Communications
- Published
- 2025-05-15
- DOI
- https://doi.org/10.1038/s41467-025-57391-8
- Citations
- 4
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 2.07
Funders
- National Research Foundation
- Ministry of Education, India